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Graphdiyne: Bridging SnO2and Perovskite in Planar Solar Cells
Abstract
The matching of charge transport layer and photoactive layer is critical in solar energy conversion devices, especially for planar perovskite solar cells based on the SnO 2 electron‐transfer layer (ETL) owing to its unmatched photogenerated electron and hole extraction rates. Graphdiyne (GDY) with multi‐roles has been incorporated to maximize the matching between SnO 2 and perovskite regarding electron extraction rate optimization and interface engineering towards both perovskite crystallization process and subsequent photovoltaic service duration. The GDY doped SnO 2 layer has fourfold improved electron mobility due to freshly formed C−O σ bond and more facilitated band alignment. The enhanced hydrophobicity inhibits heterogeneous perovskite nucleation, contributing to a high‐quality film with diminished grain boundaries and lower defect density. Also, the interfacial passivation of Pb−I anti‐site defects has been demonstrated via GDY introduction.
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Cites
Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution
Xue, Y., Huang, B., Yi, Y., Guo, Y., Zuo, Z., Li, Y., Jia, Z., Liu, H., & Li, Y. (2018) · Nature Communications · doi:10.1038/s41467-018-03896-4 · Cited by 1,011
Cited by
2D graphdiyne: An emerging carbon material
Fang, Y., Liu, Y., Qi, L., Xue, Y., & Li, Y. (2022) · Chemical Society Reviews · doi:10.1039/d1cs00592h · Cited by 520
Two-Dimensional Carbon Graphdiyne: Advances in Fundamental and Application Research
Zheng, X., Chen, S., Li, J., Wu, H., Zhang, C., Zhang, D., Chen, X., Gao, Y., He, F., Hui, L., et al. (2023) · ACS Nano · doi:10.1021/acsnano.3c03849 · Cited by 283
Self-citationBoosting hydrogen evolution reaction on few-layer graphdiyne by sp-N and B co-doping
Zhao, Y., Yang, N., Wang, C., Song, L., Yu, R., & Wang, D. (2021) · APL Materials · doi:10.1063/5.0049674 · Cited by 36
Metadata
- Authors
- Zhang, S., Si, H., Fan, W., Shi, M., Li, M., Xu, C., Zhang, Z., Liao, Q., Sattar, A., Kang, Z., & Zhang, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-05-07
- Volume
- 59
- Issue
- 28
- Pages
- 11573-11582
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3014237553
- Cited by
- 234
- References
- 1
- FWCI
- 13.33
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, S., Si, H., Fan, W., Shi, M., Li, M., Xu, C., Zhang, Z., Liao, Q., Sattar, A., Kang, Z., & Zhang, Y. (2020). Graphdiyne: Bridging SnO2and Perovskite in Planar Solar Cells. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202003502
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