The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Coordination Tunes Selectivity: Two‐Electron Oxygen Reduction on High‐Loading Molybdenum Single‐Atom Catalysts
Open accessAbstract
Single‐atom catalysts (SACs) have great potential in electrocatalysis. Their performance can be rationally optimized by tailoring the metal atoms, adjacent coordinative dopants, and metal loading. However, doing so is still a great challenge because of the limited synthesis approach and insufficient understanding of the structure–property relationships. Herein, we report a new kind of Mo SAC with a unique O,S coordination and a high metal loading over 10 wt %. The isolation and local environment was identified by high‐angle annular dark‐field scanning transmission electron microscopy and extended X‐ray absorption fine structure. The SACs catalyze the oxygen reduction reaction (ORR) via a 2 e− pathway with a high H 2 O 2 selectivity of over 95 % in 0.10 m KOH. The critical role of the Mo single atoms and the coordination structure was revealed by both electrochemical tests and theoretical calculations.
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Fei, H., Dong, J., Feng, Y., Allen, C. S., Wan, C., Volosskiy, B., Li, M., Zhao, Z., Wang, Y., Sun, H., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0008-y · Cited by 1,973
Domino electroreduction of CO2 to methanol on a molecular catalyst
Wu, Y., Jiang, Z., Lu, X., Liang, Y., & Wang, H. (2019) · Nature · doi:10.1038/s41586-019-1760-8 · Cited by 1,194
Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
Choi, C. H., Kim, M., Kwon, H. C., Cho, S. J., Yun, S., Kim, H.-T., Mayrhofer, K. J. J., Kim, H., & Choi, M. (2016) · Nature Communications · doi:10.1038/ncomms10922 · Cited by 849
Single atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
Cited by
Ma, X., Liu, H., Yang, W., Mao, G., Zheng, L., & Jiang, H.-L. (2021) · Journal of the American Chemical Society · doi:10.1021/jacs.1c05032 · Cited by 445
Jiao, L., Yang, W., Wan, G., Zhang, R., Zheng, X., Zhou, H., Yu, S., & Jiang, H. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202008787 · Cited by 412
Electrocatalysis of Single-Atom Sites: Impacts of Atomic Coordination
Lu, B., Liu, Q., & Chen, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01950 · Cited by 394
Cation‐Vacancy‐Enriched Nickel Phosphide for Efficient Electrosynthesis of Hydrogen Peroxides
Zhou, Z., Kong, Y., Tan, H., Huang, Q., Wang, C., Pei, Z., Wang, H., Liu, Y., Wang, Y., Li, S., et al. (2022) · Advanced Materials · doi:10.1002/adma.202106541 · Cited by 325
Li, Z., Yan, X., He, D., Hu, W., Younan, S., Ke, Z., Patrick, M., Xiao, X., Huang, J., Wu, H., et al. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c00759 · Cited by 83
Metadata
- Authors
- Tang, C., Jiao, Y., Shi, B., Liu, J., Xie, Z., Chen, X., Zhang, Q., & Qiao, S.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-04-07
- Volume
- 59
- Issue
- 23
- Pages
- 9171-9176
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3012441403
- Cited by
- 575
- References
- 4
- FWCI
- 18.21
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Tang, C., Jiao, Y., Shi, B., Liu, J., Xie, Z., Chen, X., Zhang, Q., & Qiao, S. (2020). Coordination Tunes Selectivity: Two‐Electron Oxygen Reduction on High‐Loading Molybdenum Single‐Atom Catalysts. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202003842
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