The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
Intrinsic Electrocatalytic Activity Regulation of M–N–C Single‐Atom Catalysts for the Oxygen Reduction Reaction
Abstract
Single‐atom catalysts (SACs) with highly active sites atomically dispersed on substrates exhibit unique advantages regarding maximum atomic efficiency, abundant chemical structures, and extraordinary catalytic performances for multiple important reactions. In particular, M–N–C SACs (M=transition metal atom) demonstrate optimal electrocatalytic activity for the oxygen reduction reaction (ORR) and have attracted extensive attention recently. Despite substantial efforts in fabricating various M–N–C SACs, the principles for regulating the intrinsic electrocatalytic activity of their active sites have not been sufficiently studied. In this Review, we summarize the regulation strategies for promoting the intrinsic electrocatalytic ORR activity of M–N–C SACs by modulation of the center metal atoms, the coordinated atoms, the environmental atoms, and the guest groups. Theoretical calculations and experimental investigations are both included to afford a comprehensive understanding of the structure–performance relationship. Finally, future directions of developing advanced M–N–C SACs for electrocatalytic ORR and other analogous reactions are proposed.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
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Cited by
Chen, Y., Gao, R., Ji, S., Li, H., Tang, K., Jiang, P., Hu, H., Zhang, Z., Hao, H., Qu, Q., et al. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202012798 · Cited by 650
Electrocatalysis of Single-Atom Sites: Impacts of Atomic Coordination
Lu, B., Liu, Q., & Chen, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01950 · Cited by 394
Xie, Y., Chen, X., Sun, K., Zhang, J., Lai, W., Liu, H., & Wang, G. (2023) · Angewandte Chemie International Edition · doi:10.1002/anie.202301833 · Cited by 197
Shen, M., Hu, W., Duan, C., Li, J., Ding, S., Zhang, L., Zhu, J., & Ni, Y. (2023) · Journal of Colloid and Interface Science · doi:10.1016/j.jcis.2022.09.035 · Cited by 67
Meng, H., Liu, X., Chen, X., Han, Y., Zhou, C., Jiang, Q., Tan, T., & Zhang, R. (2022) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2022.04.031 · Cited by 27
Metadata
- Authors
- Zhao, C., Li, B., Liu, J., & Zhang, Q.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-10-22
- Volume
- 60
- Issue
- 9
- Pages
- 4448-4463
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3016744546
- Cited by
- 725
- References
- 7
- FWCI
- 19.85
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhao, C., Li, B., Liu, J., & Zhang, Q. (2021). Intrinsic Electrocatalytic Activity Regulation of M–N–C Single‐Atom Catalysts for the Oxygen Reduction Reaction. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202003917
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