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A High Performing Zn‐Ion Battery Cathode Enabled by In Situ Transformation of V2O5 Atomic Layers
Abstract
Developing high capacity and stable cathodes is a key to successful commercialization of aqueous Zn‐ion batteries (ZIBs). Pure layered V 2 O 5 has a high theoretical capacity (585 mAh g−1), but it suffers severe capacity decay. Pre‐inserting cations into V 2 O 5 can substantially stabilize the performance, but at an expense of lowered capacity. Here we show that an atomic layer deposition derived V 2 O 5 can be an excellent ZIB cathode with high capacity and exceptional cycle stability at once. We report a rapid in situ on‐site transformation of V 2 O 5 atomic layers into Zn 3 V 2 O 7(OH)2⋅2 H 2 O (ZVO) nanoflake clusters, also a known Zn‐ion and proton intercalatable material. High concentration of reactive sites, strong bonding to the conductive substrate, nanosized thickness and binder‐free composition facilitate ionic transport and promote the best utilization of the active material. We also provide new insights into the V 2 O 5‐dissolution mechanisms for different Zn‐salt aqueous electrolytes and their implications to the cycle stability.
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Commentary: The Materials Project: A materials genome approach to accelerating materials innovation
Jain, A., Ong, S. P., Hautier, G., Chen, W., Richards, W. D., Dacek, S., Cholia, S., Gunter, D., Skinner, D., Ceder, G., et al. (2013) · APL Materials · doi:10.1063/1.4812323 · Cited by 13,094
In situ click chemistry generation of cyclooxygenase-2 inhibitors
Bhardwaj, A., Kaur, J., Wuest, M., & Wuest, F. (2017) · Nature Communications · doi:10.1038/s41467-016-0009-6 · Cited by 7,448
Cited by
Advances and Perspectives of Cathode Storage Chemistry in Aqueous Zinc-Ion Batteries
Wang, X., Zhang, Z., Xi, B., Chen, W., Jia, Y., Feng, J., & Xiong, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c01389 · Cited by 531
Zhou, M., Chen, Y., Fang, G., & Liang, S. (2022) · Energy Storage Materials · doi:10.1016/j.ensm.2021.12.011 · Cited by 316
Liu, Y., Jiang, Y., Hu, Z., Peng, J., Lai, W., Wu, D., Zuo, S., Zhang, J., Chen, B., Dai, Z., et al. (2021) · Advanced Functional Materials · doi:10.1002/adfm.202008033 · Cited by 267
Metadata
- Authors
- Lu, Y., Zhu, T., van den Bergh, W., Stefik, M., & Huang, K.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-08-06
- Volume
- 59
- Issue
- 39
- Pages
- 17004-17011
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3036898174
- Cited by
- 252
- References
- 2
- FWCI
- 13.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lu, Y., Zhu, T., van den Bergh, W., Stefik, M., & Huang, K. (2020). A High Performing Zn‐Ion Battery Cathode Enabled by In Situ Transformation of V2O5 Atomic Layers. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202006171
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