Cited by 296Electrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceNanomaterials for catalytic reactions

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Chain Mail for Catalysts

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Yu, Liang, Deng, Dehui, Bao, Xinhe·2020·Angewandte Chemie International Edition

DOI 10.1002/anie.202007604

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Abstract

Encapsulating transition‐metal nanoparticles inside carbon nanotubes (CNTs) or spheres has emerged as a novel strategy for designing highly durable nonprecious‐metal catalysts. The stable carbon layer protects the inner metal core from the destructive reaction environment and thus is described as chain mail for catalysts. Electron transfer from the active metal core to the carbon layer stimulates unique catalytic activity on the carbon surface, which has been utilized extensively in a variety of catalytic reaction systems. Here, we elaborate the underlying working principle of chain mail for catalysts as well as the key factors that determine their catalytic properties, and provide insights into the physicochemical nature of such catalyst architectures for further application of the strategy in rational catalyst design.

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Authors: Yu, L., Deng, D., & Bao, X.
Affiliations: Dalian Institute of Chemical Physics (CN)
University of Science and Technology of China (CN)
Corresponding author: Deng, Dehui
Bao, Xinhe
ORCID: Yu, Liang
Deng, Dehui
Bao, Xinhe
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2020-08-06
Volume: 59
Issue: 36
Pages: 15294-15297
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.202007604
OpenAlex: W3029614928
Cited by: 296
References: 25
Citations by year: 2026: 28 · 2025: 57 · 2024: 64 · 2023: 42 · 2022: 54 · 2021: 43 · 2020: 8
FWCI: 7.26
Type: journal article
Language: en
Open access: bronze
doi.org
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
PubMed (publishedVersion)
Funders: National Natural Science Foundation of China (21890753, 21988101, 21872140, 91845106)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
Physical Sciences › Chemistry › Organic Chemistry › Nanomaterials for catalytic reactions
Keywords: transition metal nanoparticles, carbon nanotubes, carbon encapsulation, non-noble metal catalysts, catalyst stability, electron transfer, catalyst design

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