The DOI matches its Crossref record; 9 of the 9 references it cites were found in a registry or an index.
Atomically Dispersed Reactive Centers for Electrocatalytic CO2 Reduction and Water Splitting
Open accessAbstract
Developing electrocatalytic energy conversion technologies for replacing the traditional energy source is highly expected to resolve the fossil fuel exhaustion and related environmental problems. Exploring stable and high‐efficiency electrocatalysts is of vital importance for the promotion of these technologies. Single‐atom catalysts (SACs), with atomically distributed active sites on supports, perform as emerging materials in catalysis and present promising prospects for a wide range of applications. The rationally designed near‐range coordination environment, long‐range electronic interaction and microenvironment of the coordination sphere cast huge influence on the reaction mechanism and related catalytic performance of SACs. In the current Review, some recent developments of atomically dispersed reactive centers for electrocatalytic CO 2 reduction and water splitting are well summarized. The catalytic mechanism and the underlying structure–activity relationship are elaborated based on the recent progresses of various operando investigations. Finally, by highlighting the challenges and prospects for the development of single‐atom catalysis, we hope to shed some light on the future research of SACs for the electrocatalytic energy conversion.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
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Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
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Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
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Metallic nanostructures with low dimensionality for electrochemical water splitting
Li, L., Wang, P., Shao, Q., & Huang, X. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00013b · Cited by 1,049
Large-Scale and Highly Selective CO2 Electrocatalytic Reduction on Nickel Single-Atom Catalyst
Zheng, T., Jiang, K., Ta, N., Hu, Y., Zeng, J., Liu, J., & Wang, H. (2019) · Joule · doi:10.1016/j.joule.2018.10.015 · Cited by 887
Single atom electrocatalysts supported on graphene or graphene-like carbons
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Self-citationZhang, H., Zhou, W., Lu, X. F., Chen, T., & Lou, X. W. (. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202000882 · Cited by 233
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Cited by
Single-atom catalysts for photocatalytic energy conversion
Xue, Z.-H., Luan, D., Zhang, H., & (David) Lou, X. W. (2022) · Joule · doi:10.1016/j.joule.2021.12.011 · Cited by 567
Self-citationChang, B., Pang, H., Raziq, F., Wang, S., Huang, K.-W., Ye, J., & Zhang, H. (2023) · Energy & Environmental Science · doi:10.1039/d3ee00964e · Cited by 458
Self-citationThe effect of coordination environment on the activity and selectivity of single-atom catalysts
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Wu, Z., Yang, P., Li, Q., Xiao, W., Li, Z., Xu, G., Liu, F., Jia, B., Ma, T., Feng, S., et al. (2023) · Angewandte Chemie International Edition · doi:10.1002/anie.202300406 · Cited by 226
Metadata
- Authors
- Zhang, H., Cheng, W., Luan, D., & Lou, X. W. (.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-02-24
- Volume
- 60
- Issue
- 24
- Pages
- 13177-13196
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3111845622
- Cited by
- 201
- References
- 9
- FWCI
- 6.60
- Type
- journal article
- Language
- en
- Open access
- hybrid
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