Cited by 680Advanced oxidation water treatmentElectrocatalysts for Energy ConversionPolyoxometalates: Synthesis and Applications

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Inside Cover: Mn−O Covalency Governs the Intrinsic Activity of Co‐Mn Spinel Oxides for Boosted Peroxymonosulfate Activation (Angew. Chem. Int. Ed. 1/2021)

Guo, Zhi‐Yan, Li, Chen‐Xuan, Gao, Miao, Han, Xiao, Zhang, Ying‐Jie, Zhang, Wen‐Jun, Li, Wen‐Wei·2021·Angewandte Chemie International Edition

DOI 10.1002/anie.202014556

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Abstract

Bimetallic spinel oxides are efficient catalysts for peroxymonosulfate (PMS) activation but the catalytic mechanism is unclear. The critical role of Mn−O covalency in determining the intrinsic activity of Co3−xMnxO4 and a new mechanism of Co–Mn synergy are revealed by Wen-Wei Li and co-workers in their Research Article on page 274. Co strengthens Mn−O covalency in the octahedral configuration of Co3−xMnxO4, which lowers the charge transfer energy of the MnOh–PMS interaction and drastically accelerates MnVI/MnIII redox cycling.

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Authors: Guo, Z., Li, C., Gao, M., Han, X., Zhang, Y., Zhang, W., & Li, W.
Affiliations: Department of Environmental Science and Engineering University of Science & Technology of China Hefei 230026 China
University of Science and Technology of China (CN)
Department of Materials Science and Engineering City University of Hong Kong, Hong Kong SAR China
Corresponding author: Li, Wen‐Wei
ORCID: Li, Chen‐Xuan
Gao, Miao
Han, Xiao
Li, Wen‐Wei
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2020-11-12
Volume: 60
Issue: 1
Pages: 2-2
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.202014556
OpenAlex: W3118166060
Cited by: 680
References: 0
Citations by year: 2026: 9 · 2025: 25 · 2024: 51 · 2023: 90 · 2022: 177 · 2021: 327 · 2020: 1
FWCI: 45.59
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
Topics: Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › Polyoxometalates: Synthesis and Applications
Keywords: peroxymonosulfate activation, catalytic mechanism, charge transfer energy, advanced oxidation processes

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Inside Cover: Mn−O Covalency Governs the Intrinsic Activity of Co‐Mn Spinel Oxides for Boosted Peroxymonosulfate Activation (Angew. Chem. Int. Ed. 1/2021)

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