The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Boosting Zinc Electrode Reversibility in Aqueous Electrolytes by Using Low‐Cost Antisolvents
Abstract
Antisolvent addition has been widely studied in crystallization in the pharmaceutical industries by breaking the solvation balance of the original solution. Here we report a similar antisolvent strategy to boost Zn reversibility via regulation of the electrolyte on a molecular level. By adding for example methanol into ZnSO 4 electrolyte, the free water and coordinated water in Zn 2+solvation sheath gradually interact with the antisolvent, which minimizes water activity and weakens Zn 2+solvation. Concomitantly, dendrite‐free Zn deposition occurs via change in the deposition orientation, as evidenced by in situ optical microscopy. Zn reversibility is significantly boosted in antisolvent electrolyte of 50 % methanol by volume (Anti‐M‐50 %) even under harsh environments of −20 °C and 60 °C. Additionally, the suppressed side reactions and dendrite‐free Zn plating/stripping in Anti‐M‐50 % electrolyte significantly enhance performance of Zn/polyaniline coin and pouch cells. We demonstrate this low‐cost strategy can be readily generalized to other solvents, indicating its practical universality. Results will be of immediate interest and benefit to a range of researchers in electrochemistry and energy storage.
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Double-slit photoelectron interference in strong-field ionization of the neon dimer
Kunitski, M., Eicke, N., Huber, P., Köhler, J., Zeller, S., Voigtsberger, J., Schlott, N., Henrichs, K., Sann, H., Trinter, F., et al. (2019) · Nature Communications · doi:10.1038/s41467-018-07882-8 · Cited by 8,162
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
SARS-CoV-2 proteome microarray for global profiling of COVID-19 specific IgG and IgM responses
Jiang, H.-W., Li, Y., Zhang, H.-N., Wang, W., Yang, X., Qi, H., Li, H., Men, D., Zhou, J., & Tao, S.-C. (2020) · Nature Communications · doi:10.1038/s41467-020-17488-8 · Cited by 329
Cited by
Huang, S., Hou, L., Li, T., Jiao, Y., & Wu, P. (2022) · Advanced Materials · doi:10.1002/adma.202110140 · Cited by 595
Recent Progress on Zn Anodes for Advanced Aqueous Zinc‐Ion Batteries
Nie, C., Wang, G., Wang, D., Wang, M., Gao, X., Bai, Z., Wang, N., Yang, J., Xing, Z., & Dou, S. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202300606 · Cited by 561
Gel polymer electrolytes for rechargeable batteries toward wide-temperature applications
Zhou, X., Zhou, Y., Yu, L., Qi, L., Oh, K.-S., Hu, P., Lee, S.-Y., & Chen, C. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00551h · Cited by 333
Designing Electrolyte Structure to Suppress Hydrogen Evolution Reaction in Aqueous Batteries
Nian, Q., Zhang, X., Feng, Y., Liu, S., Sun, T., Zheng, S., Ren, X., Tao, Z., Zhang, D., & Chen, J. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.1c00833 · Cited by 303
Metadata
- Authors
- Hao, J., Yuan, L., Ye, C., Chao, D., Davey, K., Guo, Z., & Qiao, S.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-02-24
- Volume
- 60
- Issue
- 13
- Pages
- 7366-7375
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3132344615
- Cited by
- 935
- References
- 3
- FWCI
- 48.89
- Type
- journal article
- Language
- en
- Open access
- closed
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