The DOI matches its Crossref record; 58 of the 58 references it cites were found in a registry or an index.
Intrinsic Electrocatalytic Activity for Oxygen Evolution of Crystalline 3d‐Transition Metal Layered Double Hydroxides
Open accessAbstract
Layered double hydroxides (LDHs) are among the most active and studied catalysts for the oxygen evolution reaction (OER) in alkaline electrolytes. However, previous studies have generally either focused on a small number of LDHs, applied synthetic routes with limited structural control, or used non‐intrinsic activity metrics, thus hampering the construction of consistent structure–activity‐relations. Herein, by employing new individually developed synthesis strategies with atomic structural control, we obtained a broad series of crystalline α‐M A(II)M B(III) LDH and β‐M A(OH)2 electrocatalysts (M A=Ni, Co, and M B=Co, Fe, Mn). We further derived their intrinsic activity through electrochemical active surface area normalization, yielding the trend NiFe LDH > CoFe LDH > Fe‐free Co‐containing catalysts > Fe‐Co‐free Ni‐based catalysts. Our theoretical reactivity analysis revealed that these intrinsic activity trends originate from the dual‐metal‐site nature of the reaction centers, which lead to composition‐dependent synergies and diverse scaling relationships that may be used to design catalysts with improved performance.
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Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
A Perovskite Oxide Optimized for Oxygen Evolution Catalysis from Molecular Orbital Principles
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Self-citationIdentification of Highly Active Fe Sites in (Ni,Fe)OOH for Electrocatalytic Water Splitting
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A highly active and stable IrO x /SrIrO 3 catalyst for the oxygen evolution reaction
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Cited by
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
Self-citationJeon, S. S., Kang, P. W., Klingenhof, M., Lee, H., Dionigi, F., & Strasser, P. (2023) · ACS Catalysis · doi:10.1021/acscatal.2c04452 · Cited by 316
Self-citationiR Compensation for Electrocatalysis Studies: Considerations and Recommendations
Zheng, W. (2023) · ACS Energy Letters · doi:10.1021/acsenergylett.3c00366 · Cited by 285
Jiang, W., Faid, A. Y., Gomes, B. F., Galkina, I., Xia, L., Lobo, C. M. S., Desmau, M., Borowski, P., Hartmann, H., Maljusch, A., et al. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202203520 · Cited by 161
Pham, T. M., Plevova, M., Bartling, S., Rockstroh, N., Springer, A., Slabon, A., Hnat, J., Surkus, A.-E., & Francke, R. (2024) · Journal of Catalysis · doi:10.1016/j.jcat.2024.115675 · Cited by 9
Metadata
- Authors
- Dionigi, F., Zhu, J., Zeng, Z., Merzdorf, T., Sarodnik, H., Gliech, M., Pan, L., Li, W., Greeley, J., & Strasser, P.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-05-26
- Volume
- 60
- Issue
- 26
- Pages
- 14446-14457
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3156253791
- Cited by
- 300
- References
- 58
- FWCI
- 9.37
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Dionigi, F., Zhu, J., Zeng, Z., Merzdorf, T., Sarodnik, H., Gliech, M., Pan, L., Li, W., Greeley, J., & Strasser, P. (2021). Intrinsic Electrocatalytic Activity for Oxygen Evolution of Crystalline 3d‐Transition Metal Layered Double Hydroxides. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202100631
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