The DOI matches its Crossref record; 44 of the 44 references it cites were found in a registry or an index.
High‐Performance Electrochemical NO Reduction into NH3 by MoS2 Nanosheet
Abstract
Electrochemical reduction of NO not only offers an attractive alternative to the Haber–Bosch process for ambient NH 3 production but mitigates the human‐caused unbalance of nitrogen cycle. Herein, we report that MoS 2 nanosheet on graphite felt (MoS 2/GF) acts as an efficient and robust 3D electrocatalyst for NO‐to‐NH 3 conversion. In acidic electrolyte, such MoS 2/GF attains a maximal Faradaic efficiency of 76.6 % and a large NH 3 yield of up to 99.6 μmol cm−2 h−1. Using MoS 2 nanosheet‐loaded carbon paper as the cathode, a proof‐of‐concept device of Zn‐NO battery was assembled to deliver a discharge power density of 1.04 mW cm−2 and an NH 3 yield of 411.8 μg h−1 mg cat.−1. Calculations reveal that the positively charged Mo‐edge sites facilitate NO adsorption/activation via an acceptance–donation mechanism and disfavor the binding of protons and the coupling of N−N bond.
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Cites
A fast and robust algorithm for Bader decomposition of charge density
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An Earth-system perspective of the global nitrogen cycle
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Nitrogen Cycle Electrocatalysis
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Ammonia for hydrogen storage: challenges and opportunities
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Recent Advances and Challenges of Electrocatalytic N2Reduction to Ammonia
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Cited by
Electrochemical Reduction of Gaseous Nitrogen Oxides on Transition Metals at Ambient Conditions
Ko, B. H., Hasa, B., Shin, H., Zhao, Y., & Jiao, F. (2022) · Journal of the American Chemical Society · doi:10.1021/jacs.1c10535 · Cited by 280
Metadata
- Authors
- Zhang, L., Liang, J., Wang, Y., Mou, T., Lin, Y., Yue, L., Li, T., Liu, Q., Luo, Y., Li, N., Tang, B., Liu, Y., Gao, S., Alshehri, A. A., Guo, X., Ma, D., & Sun, X.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-10-27
- Volume
- 60
- Issue
- 48
- Pages
- 25263-25268
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3200149094
- Cited by
- 325
- References
- 44
- FWCI
- 11.24
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, L., Liang, J., Wang, Y., Mou, T., Lin, Y., Yue, L., Li, T., Liu, Q., Luo, Y., Li, N., Tang, B., Liu, Y., Gao, S., Alshehri, A. A., Guo, X., Ma, D., & Sun, X. (2021). High‐Performance Electrochemical NO Reduction into NH3 by MoS2 Nanosheet. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202110879
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