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Selective Electrooxidation of Biomass‐Derived Alcohols to Aldehydes in a Neutral Medium: Promoted Water Dissociation over a Nickel‐Oxide‐Supported Ruthenium Single‐Atom Catalyst
Abstract
The biomass‐derived alcohol oxidation reaction (BDAOR) holds great promise for sustainable production of chemicals. However, selective electrooxidation of alcohols to value‐added aldehyde compounds is still challenging. Herein, we report the electrocatalytic BDAORs to selectively produce aldehydes using single‐atom ruthenium on nickel oxide (Ru 1‐NiO) as a catalyst in the neutral medium. For electrooxidation of 5‐hydroxymethylfurfural (HMF), Ru 1‐NiO exhibits a low potential of 1.283 V at 10 mA cm−2, and an optimal 2,5‐diformylfuran (DFF) selectivity of 90 %. Experimental studies reveal that the neutral electrolyte plays a critical role in achieving a high aldehyde selectivity, and the single‐atom Ru boosts HMF oxidation in the neutral medium by promoting water dissociation to afford OH*. Furthermore, Ru 1‐NiO can be extended to selective electrooxidation of a series of biomass‐derived alcohols to corresponding aldehydes, which are conventionally difficult to obtain in the alkaline medium.
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Yang, Y., & Mu, T. (2021) · Green Chemistry · doi:10.1039/d1gc00914a · Cited by 539
Cited by
Heterogeneous‐Interface‐Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation
Zhou, P., Lv, X., Tao, S., Wu, J., Wang, H., Wei, X., Wang, T., Zhou, B., Lu, Y., Frauenheim, T., et al. (2022) · Advanced Materials · doi:10.1002/adma.202204089 · Cited by 570
Zhou, P., Hai, G., Zhao, G., Li, R., Huang, X., Lu, Y., & Wang, G. (2023) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2023.122364 · Cited by 259
Yang, Z., Wang, S., Wei, C., Chen, L., Xue, Z., & Mu, T. (2024) · Energy & Environmental Science · doi:10.1039/d3ee04543a · Cited by 169
Electrocatalysts for the Oxygen Evolution Reaction: Mechanism, Innovative Strategies, and Beyond
Wen, N., Jiao, X., Xia, Y., & Chen, D. (2023) · Materials Chemistry Frontiers · doi:10.1039/d3qm00423f · Cited by 104
Mu, X., Zhang, X., Chen, Z., Gao, Y., Yu, M., Chen, D., Pan, H., Liu, S., Wang, D., & Mu, S. (2024) · Nano Letters · doi:10.1021/acs.nanolett.3c04690 · Cited by 101
Metadata
- Authors
- Ge, R., Wang, Y., Li, Z., Xu, M., Xu, S., Zhou, H., Ji, K., Chen, F., Zhou, J., & Duan, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2022-02-25
- Volume
- 61
- Issue
- 19
- Pages
- e202200211-e202200211
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4213364019
- Cited by
- 449
- References
- 1
- FWCI
- 15.86
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Ge, R., Wang, Y., Li, Z., Xu, M., Xu, S., Zhou, H., Ji, K., Chen, F., Zhou, J., & Duan, H. (2022). Selective Electrooxidation of Biomass‐Derived Alcohols to Aldehydes in a Neutral Medium: Promoted Water Dissociation over a Nickel‐Oxide‐Supported Ruthenium Single‐Atom Catalyst. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202200211
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