The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Structurally Disordered RuO2 Nanosheets with Rich Oxygen Vacancies for Enhanced Nitrate Electroreduction to Ammonia
Abstract
Electrochemical reduction of nitrate pollutants to ammonia has emerged as an attractive alternative for ammonia synthesis. Currently, many strategies have been developed for enhancing nitrate reduction to ammonia (NRA) efficiency, but the influence of the degree of structural disorder is still unexplored. Here, carbon‐supported RuO 2 nanosheets with adjustable crystallinity are synthesized by a facile molten salt method. The as‐synthesized amorphous RuO 2 displays high ammonia Faradaic efficiency (97.46 %) and selectivity (96.42 %), greatly outperforming the crystalline counterparts. The disordered structure with abundant oxygen vacancies is revealed to modulate the d‐band center and hydrogen affinity, thus lowering the energy of the potential‐determining step (NH 2*→NH 3*).
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Cites
Bao, J., Zhang, X., Fan, B., Zhang, J., Zhou, M., Yang, W., Hu, X., Wang, H., Pan, B., & Xie, Y. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201502226 · Cited by 1,428
Self-citationKibsgaard, J., Tsai, C., Chan, K., Benck, J. D., Nørskov, J. K., Abild-Pedersen, F., & Jaramillo, T. F. (2015) · Energy & Environmental Science · doi:10.1039/c5ee02179k · Cited by 979
Zhang, C., Huang, Y., Yu, Y., Zhang, J., Zhuo, S., & Zhang, B. (2017) · Chemical Science · doi:10.1039/c6sc05687c · Cited by 273
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Cited by
Alloying of Cu with Ru Enabling the Relay Catalysis for Reduction of Nitrate to Ammonia
Gao, W., Xie, K., Xie, J., Wang, X., Zhang, H., Chen, S., Wang, H., Li, Z., & Li, C. (2023) · Advanced Materials · doi:10.1002/adma.202202952 · Cited by 532
Zhou, J., Wen, M., Huang, R., Wu, Q., Luo, Y., Tian, Y., Wei, G., & Fu, Y. (2023) · Energy & Environmental Science · doi:10.1039/d2ee04095f · Cited by 398
Construction of Zn-doped RuO2 nanowires for efficient and stable water oxidation in acidic media
Zhang, D., Li, M., Yong, X., Song, H., Waterhouse, G. I. N., Yi, Y., Xue, B., Zhang, D., Liu, B., & Lu, S. (2023) · Nature Communications · doi:10.1038/s41467-023-38213-1 · Cited by 380
Liu, K., Li, H., Xie, M., Wang, P., Jin, Z., Liu, Y., Zhou, M., Li, P., & Yu, G. (2024) · Journal of the American Chemical Society · doi:10.1021/jacs.4c00429 · Cited by 369
Self-citationProgress of Amorphous Catalysts for an Acidic Oxygen Evolution Reaction
Wei, L., Yang, F., Cai, W., & Feng, L. (2025) · Energy & Fuels · doi:10.1021/acs.energyfuels.5c02796 · Cited by 15
Metadata
- Authors
- Wang, Y., Li, H., Zhou, W., Zhang, X., Zhang, B., & Yu, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2022-03-11
- Volume
- 61
- Issue
- 19
- Pages
- e202202604-e202202604
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4214568875
- Cited by
- 366
- References
- 3
- FWCI
- 14.04
- Type
- journal article
- Language
- en
- Open access
- closed
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