The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
A Site Distance Effect Induced by Reactant Molecule Matchup in Single‐Atom Catalysts for Fenton‐Like Reactions
Abstract
Understanding the site interaction nature of single‐atom catalysts (SACs), especially densely populated SACs, is vital for their application to various catalytic reactions. Herein, we report a site distance effect, which emphasizes how well the distance of the adjacent copper atoms (denoted as dCu1−Cu1) matches with the reactant peroxydisulfate (PDS) molecular size to determine the Fenton‐like reaction reactivity on the carbon‐supported SACs. The optimized dCu1−Cu1 in the range of 5–6 Å, which matches the molecular size of PDS, endows the catalyst with a nearly two times higher turnover frequency than that of dCu1−Cu1 beyond this range, accordingly achieving record‐breaking kinetics for the oxidation of emerging organic contaminants. Further studies suggest that this site distance effect originates from the alteration of PDS adsorption to a dual‐site structure on Cu 1−Cu 1 sites when dCu1−Cu1 falls within 5–6 Å, significantly enhancing the interfacial charge transfer and consequently resulting in the most efficient catalyst for PDS activation so far.
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Cites
Yun, E.-T., Lee, J. H., Kim, J., Park, H.-D., & Lee, J. (2018) · Environmental Science & Technology · doi:10.1021/acs.est.8b00959 · Cited by 1,175
Zhang, T., Chen, Y., Wang, Y., Le Roux, J., Yang, Y., & Croué, J.-P. (2014) · Environmental Science & Technology · doi:10.1021/es501218f · Cited by 798
Cited by
Liu, H.-Z., Shu, X.-X., Huang, M., Wu, B.-B., Chen, J.-J., Wang, X.-S., Li, H.-L., & Yu, H.-Q. (2024) · Nature Communications · doi:10.1038/s41467-024-46739-1 · Cited by 396
Microenvironment Engineering of Single/Dual‐Atom Catalysts for Electrocatalytic Application
Gao, Y., Liu, B., & Wang, D. (2023) · Advanced Materials · doi:10.1002/adma.202209654 · Cited by 319
Self-citationHuang, B., Wu, Z., Wang, X., Song, X., Zhou, H., Zhang, H., Zhou, P., Liu, W., Xiong, Z., & Lai, B. (2023) · Environmental Science & Technology · doi:10.1021/acs.est.3c05509 · Cited by 281
Self-citationLong‐Range Interactions in Diatomic Catalysts Boosting Electrocatalysis
Li, W., Yang, J., & Wang, D. (2022) · Angewandte Chemie International Edition · doi:10.1002/anie.202213318 · Cited by 270
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Metadata
- Authors
- Wang, B., Cheng, C., Jin, M., He, J., Zhang, H., Ren, W., Li, J., Wang, D., & Li, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2022-07-08
- Volume
- 61
- Issue
- 33
- Pages
- e202207268-e202207268
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4283156879
- Cited by
- 287
- References
- 2
- FWCI
- 17.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, B., Cheng, C., Jin, M., He, J., Zhang, H., Ren, W., Li, J., Wang, D., & Li, Y. (2022). A Site Distance Effect Induced by Reactant Molecule Matchup in Single‐Atom Catalysts for Fenton‐Like Reactions. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202207268
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