The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Amorphous Mo‐doped NiS0.5Se0.5 Nanosheets@Crystalline NiS0.5Se0.5 Nanorods for High Current‐density Electrocatalytic Water Splitting in Neutral Media
Abstract
It is vitally important to develop highly active, robust and low‐cost transition metal‐based electrocatalysts for overall water splitting in neutral solution especially at large current density. In this work, amorphous Mo‐doped NiS 0.5 Se 0.5 nanosheets@crystalline NiS 0.5 Se 0.5 nanorods (Am−Mo−NiS 0.5 Se 0.5) was synthesized using a facil one‐step strategy. In phosphate buffer saline solution, the Am−Mo−NiS 0.5 Se 0.5 shows tiny overpotentials of 48 and 209 mV for hydrogen evolution reaction (HER), 238 and 514 mV for oxygen evolution reaction (OER) at 10 and 1000 mA cm−2, respectively. Moreover, Am−Mo−NiS 0.5 Se 0.5 delivers excellent stability for at least 300 h without obvious degradation. Theoretical calculations revealed that the Ni sites in the defect‐rich amorphous structure of Am−Mo−NiS 0.5 Se 0.5 owns higher electron state density and strengthened the binding energy of H 2 O, which will optimize H adsorption/desorption energy barriers and reduce the adsorption energy of OER determining step.
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Cites
Improving the hydrogen oxidation reaction rate by promotion of hydroxyl adsorption
Strmcnik, D., Uchimura, M., Wang, C., Subbaraman, R., Danilovic, N., van der Vliet, D., Paulikas, A. P., Stamenkovic, V. R., & Markovic, N. M. (2013) · Nature Chemistry · doi:10.1038/nchem.1574 · Cited by 1,426
Jiang, K., Liu, B., Luo, M., Ning, S., Peng, M., Zhao, Y., Lu, Y.-R., Chan, T.-S., de Groot, F. M. F., & Tan, Y. (2019) · Nature Communications · doi:10.1038/s41467-019-09765-y · Cited by 670
Zhang, L., Han, L., Liu, H., Liu, X., & Luo, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201706921 · Cited by 532
Ultrahigh-current-density niobium disulfide catalysts for hydrogen evolution
Yang, J., Mohmad, A. R., Wang, Y., Fullon, R., Song, X., Zhao, F., Bozkurt, I., Augustin, M., Santos, E. J. G., Shin, H. S., et al. (2019) · Nature Materials · doi:10.1038/s41563-019-0463-8 · Cited by 401
Self-citationLin, Q., Guo, D., Zhou, L., Yang, L., Jin, H., Li, J., Fang, G., Chen, X., & Wang, S. (2022) · ACS Nano · doi:10.1021/acsnano.2c07588 · Cited by 95
Cited by
Defect engineering of two-dimensional materials for advanced energy conversion and storage
Liu, F., & Fan, Z. (2023) · Chemical Society Reviews · doi:10.1039/d2cs00931e · Cited by 417
Electrocatalysts for the Oxygen Evolution Reaction: Mechanism, Innovative Strategies, and Beyond
Wen, N., Jiao, X., Xia, Y., & Chen, D. (2023) · Materials Chemistry Frontiers · doi:10.1039/d3qm00423f · Cited by 104
Li, Y., Feng, A., Dai, L., Xi, B., An, X., Xiong, S., & An, C. (2024) · Advanced Functional Materials · doi:10.1002/adfm.202316296 · Cited by 91
Metadata
- Authors
- Wang, Y., Li, X., Huang, Z., Wang, H., Chen, Z., Zhang, J., Zheng, X., Deng, Y., & Hu, W.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2023-01-02
- Volume
- 62
- Issue
- 6
- Pages
- e202215256-e202215256
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4310642939
- Cited by
- 185
- References
- 5
- FWCI
- 7.10
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, Y., Li, X., Huang, Z., Wang, H., Chen, Z., Zhang, J., Zheng, X., Deng, Y., & Hu, W. (2023). Amorphous Mo‐doped NiS0.5Se0.5 Nanosheets@Crystalline NiS0.5Se0.5 Nanorods for High Current‐density Electrocatalytic Water Splitting in Neutral Media. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202215256
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