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Analysis of nonsolvent–solvent–polymer phase diagrams and their relevance to membrane formation modeling
Open accessAbstract
Calculations have been carried out, based on Flory–Huggins solution theory, to analyze the behavior of the ternary nonsolvent–solvent–polymer phase diagram for typical membrane‐forming systems. Consideration is given to the behavior of the spinodal as well as binodal curves, tie‐line slopes, and critical points as a function of various parameters, most especially those related to the concentration dependency of the interaction parameters. Implications regarding membrane structure formation are discussed, and the suitability of different functional forms for the interaction parameter concentration dependence is also analyzed. The net result of these calculations is to demonstrate the importance of the various parameters in controlling the phase‐diagram behavior and particularly to show the critical role of the concentration dependence of the solvent–polymer interaction parameter in affecting the nature of the miscibility gap.
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Cited by
Guillen, G. R., Pan, Y., Li, M., & Hoek, E. M. V. (2011) · Industrial & Engineering Chemistry Research · doi:10.1021/ie101928r · Cited by 1,521
Effect of PEG additive on membrane formation by phase inversion
Kim, J.-H., & Lee, K.-H. (1998) · Journal of Membrane Science · doi:10.1016/s0376-7388(97)00224-x · Cited by 567
Morphology of Porous and Wrinkled Fibers of Polystyrene Electrospun from Dimethylformamide
Pai, C.-L., Boyce, M. C., & Rutledge, G. C. (2009) · Macromolecules · doi:10.1021/ma802529h · Cited by 260
Phase inversion dynamics of PLGA solutions related to drug delivery
Graham, P. D., Brodbeck, K. J., & McHugh, A. J. (1999) · Journal of Controlled Release · doi:10.1016/s0168-3659(98)00158-8 · Cited by 222
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Metadata
- Authors
- Yilmaz, L., & McHugh, A. J.
- Venue
- Journal of Applied Polymer Science
- Publisher
- Wiley
- Published
- 1986-03
- Volume
- 31
- Issue
- 4
- Pages
- 997-1018
- ISSN
- 0021-8995 (ISSN-L)
- 1097-4628
- OpenAlex
- W2047570665
- Cited by
- 253
- References
- 0
- FWCI
- 6.55
- Type
- journal article
- Language
- en
- Open access
- green
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- Yilmaz, L., & McHugh, A. J. (1986). Analysis of nonsolvent–solvent–polymer phase diagrams and their relevance to membrane formation modeling. Journal of Applied Polymer Science. https://doi.org/10.1002/app.1986.070310404
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