Colloidal Templating Fabrication of Aluminum‐Organophosphonate Films Using High Molecular Weight PS‐b‐PEO
Abstract
High molecular weight polystyrene-block-poly(ethylene oxide) diblock copolymer (PS-b-PEO) is utilized as colloidal spheres in the presence of water. Adequately thick films with multilayers of spherical macropores are fabricated in one-pot under highly concentrated conditions of PS-b-PEO. The frameworks are constructed using aluminum organophosphonate as a complicated hybrid component. The macropores (30-200 nm) are homogeneously distributed over the entire films and pore windows between the macropores are tunable (up to nearly 10 nm) by changing the relative amount of PS-b-PEO in the precursor solutions.
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Aluminum-organophosphonate films with tunable macropores (30-200 nm) were synthesized via ultra-high molecular weight PEO-b-PS (250,000 g/mol) templates, though the resulting material exhibited a relatively disordered mesostructure.
“In another case, aluminum-organophosphonate films with tunable macropores (30–200 nm) were synthesized via ultra-high molecular weight PEO-b-PS (250,000 g/mol) templates, though the resulting material exhibited a relatively disordered mesostructure [157].”
From Block Copolymers: Synthesis, Self-Assembly, and Applications (2017) · cites this paper as [157]
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References 64 · Cited by 17
- Authors
- Kimura, T.
- Affiliations
- National Institute of Advanced Industrial Science and Technology (JP)
- Corresponding author
- Kimura, Tatsuo
- ORCID
- Kimura, Tatsuo
- Venue
- Chemistry – An Asian Journal
- Publisher
- Wiley
- Published
- 2011-09-06
- Volume
- 6
- Issue
- 12
- Pages
- 3236-3242
- ISSN
- 1861-471X (ISSN-L)
- 1861-4728
- OpenAlex
- W1973677612
- Cited by
- 17
- References
- 64
- Citations by year
- 2022: 1 · 2019: 1 · 2017: 1 · 2016: 2 · 2015: 3 · 2014: 3 · 2013: 1 · 2012: 5
- FWCI
- 1.41
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Chemistry - An Asian Journal (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › Block Copolymer Self-Assembly
- Physical Sciences › Materials Science › Materials Chemistry › Mesoporous Materials and Catalysis
- Physical Sciences › Chemistry › Organic Chemistry › Advanced Polymer Synthesis and Characterization
- Keywords
- colloidal templating, polystyrene-block-poly(ethylene oxide), macroporous films, hybrid materials, one-pot synthesis, pore size control, multilayer films, block copolymer self-assembly
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