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Enhanced Fluorescence of Remote Functionalized Diaminodicyanoquinodimethanes in the Solid State and Fluorescence Switching in a Doped Polymer by Solvent Vapors
Abstract
Remote functionalized zwitterionic diaminodicyanoquinodimethanes are found to exhibit a dramatic enhancement of light emission in the solid state and when doped in polymer films, as compared to the solution state. Crystal structure analysis of prototypical molecules reveals the role of the remote functionality in the solid state molecular organization. Semiempirical quantum chemical computations provide a viable model to explain the interesting phenomenon of fluorescence enhancement as arising from the inhibition of geometry relaxation of the vertical excited state to a nonemitting state. The reversible switching of a doped polymer film fluorescence triggered by solvent vapors is demonstrated.
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Citations
Cites
Aggregation-induced emission of 1-methyl-1,2,3,4,5-pentaphenylsilole
Luo, J., Xie, Z., Lam, J. W. Y., Cheng, L., Tang, B. Z., Chen, H., Qiu, C., Kwok, H. S., Zhan, X., Liu, Y., et al. (2001) · Chemical Communications · doi:10.1039/b105159h · Cited by 8,358
Cited by
Hong, Y., Lam, J. W. Y., & Tang, B. Z. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15113d · Cited by 6,363
Dong, Y., Lam, J. W. Y., Qin, A., Li, Z., Sun, J., Sung, H. H.-Y., Williams, I. D., & Tang, B. Z. (2007) · Chem. Commun. · doi:10.1039/b613157c · Cited by 428
Li, Z., Dong, Y., Mi, B., Tang, Y., Häussler, M., Tong, H., Dong, Y., Lam, J. W. Y., Ren, Y., Sung, H. H. Y., et al. (2005) · The Journal of Physical Chemistry B · doi:10.1021/jp0503462 · Cited by 360
Anthony, S. P. (2012) · ChemPlusChem · doi:10.1002/cplu.201200073 · Cited by 278
Ma, J., Lin, T., Pan, X., & Wang, W. (2014) · Chemistry of Materials · doi:10.1021/cm501590w · Cited by 59
Metadata
- Authors
- Jayanty, S., & Radhakrishnan, T. P.
- Venue
- Chemistry – A European Journal
- Publisher
- Wiley
- Published
- 2004-02-02
- Volume
- 10
- Issue
- 3
- Pages
- 791-797
- ISSN
- 0947-6539 (ISSN-L)
- 1521-3765
- OpenAlex
- W2117907852
- Cited by
- 166
- References
- 1
- FWCI
- 4.58
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jayanty, S., & Radhakrishnan, T. P. (2004). Enhanced Fluorescence of Remote Functionalized Diaminodicyanoquinodimethanes in the Solid State and Fluorescence Switching in a Doped Polymer by Solvent Vapors. Chemistry – A European Journal. https://doi.org/10.1002/chem.200305123
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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