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Design and Generation of Extended Zeolitic Metal–Organic Frameworks (ZMOFs): Synthesis and Crystal Structures of Zinc(II) Imidazolate Polymers with Zeolitic Topologies
Abstract
Attempts to create metal–organic frameworks (MOFs) with zeolitic topologies, metal (zinc(II) and cobalt(II)) imidazolates have repeatedly been used as the metal–organic motifs of inorganic silicate analogues. By modulating the synthetic strategy based on the solvothermal and liquid diffusion method, seven further MOFs (including at least three zeolitic MOFs) of zinc(II) imidazolates, [Zn(im)2⋅x G] (G=guest molecule, x=0.2–1) 1 a–7 a, have been successfully synthesized. Of these, 1 a–3 a are isostructural with the previously reported cobalt analogues 1 b–3 b, respectively, while 4 a–7 a are new members of the metal imidazolate MOF family. Complex 4 a exhibits a structure related to silicate CaAl 2 Si 2 O 8 of CrB 4 topology, but with a higher network symmetry; complex 5 a has a structure with zeolitic DFT topology that was discovered in zeolite‐related materials of DAF‐2, UCSB‐3, and UCSB‐3GaGe; complex 6 a demonstrates an unprecedented zeolite‐like topology with one dimensional channels with 10‐rings; and 7 a displays a structure of natural zeolite GIS (gismondine) topology. All of these polymorphous MOFs were created only by using certain solvents as structure‐directing agents (SDAs). Further extensive metal–organic frameworks with zeolitic topologies can be envisaged if other solvents were to be used.
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Eddaoudi, M., Sava, D. F., Eubank, J. F., Adil, K., & Guillerm, V. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00230j · Cited by 773
Tan, J. C., & Cheetham, A. K. (2011) · Chemical Society Reviews · doi:10.1039/c0cs00163e · Cited by 762
Zeolitic imidazolate framework-8 as efficient pH-sensitive drug delivery vehicle
Sun, C.-Y., Qin, C., Wang, X.-L., Yang, G.-S., Shao, K.-Z., Lan, Y.-Q., Su, Z.-M., Huang, P., Wang, C.-G., & Wang, E.-B. (2012) · Dalton Transactions · doi:10.1039/c2dt30357d · Cited by 710
Tan, J. C., Bennett, T. D., & Cheetham, A. K. (2010) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1003205107 · Cited by 552
Adsorption of CO2, CH4, and N2 on Zeolitic Imidazolate Frameworks: Experiments and Simulations
Pérez‐Pellitero, J., Amrouche, H., Siperstein, F. R., Pirngruber, G., Nieto‐Draghi, C., Chaplais, G., Simon‐Masseron, A., Bazer‐Bachi, D., Peralta, D., & Bats, N. (2010) · Chemistry – A European Journal · doi:10.1002/chem.200902144 · Cited by 417
Metadata
- Authors
- Tian, Y., Zhao, Y., Chen, Z., Zhang, G., Weng, L., & Zhao, D.
- Venue
- Chemistry – A European Journal
- Publisher
- Wiley
- Published
- 2007-05-04
- Volume
- 13
- Issue
- 15
- Pages
- 4146-4154
- ISSN
- 0947-6539 (ISSN-L)
- 1521-3765
- OpenAlex
- W2096051064
- Cited by
- 384
- References
- 25
- FWCI
- 16.13
- Type
- journal article
- Language
- en
- Open access
- closed
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- Tian, Y., Zhao, Y., Chen, Z., Zhang, G., Weng, L., & Zhao, D. (2007). Design and Generation of Extended Zeolitic Metal–Organic Frameworks (ZMOFs): Synthesis and Crystal Structures of Zinc(II) Imidazolate Polymers with Zeolitic Topologies. Chemistry – A European Journal. https://doi.org/10.1002/chem.200700181
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