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Water Stable Zr–Benzenedicarboxylate Metal–Organic Frameworks as Photocatalysts for Hydrogen Generation
Abstract
The Zr‐containing metal–organic frameworks (MOFs) formed by terephthalate (UiO‐66) and 2‐aminoterephthalate ligands [UiO‐66(NH 2)] are two notably water‐resistant MOFs that exhibit photocatalytic activity for hydrogen generation in methanol or water/methanol upon irradiation at wavelength longer than 300 nm. The apparent quantum yield for H 2 generation using monochromatic light at 370 nm in water/methanol 3:1 was of 3.5 % for UiO‐66(NH 2). Laser‐flash photolysis has allowed detecting for UiO‐66 and UiO‐66(NH 2) the photochemical generation of a long lived charge separated state whose decay is not complete 300 μs after the laser flash. Our finding and particularly the influence of the amino group producing a bathochromic shift in the optical spectrum without altering the photochemistry shows promises for the development of more efficient MOFs for water splitting.
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Cited by
Valenzano, L., Civalleri, B., Chavan, S., Bordiga, S., Nilsen, M. H., Jakobsen, S., Lillerud, K. P., & Lamberti, C. (2011) · Chemistry of Materials · doi:10.1021/cm1022882 · Cited by 1,919
Xu, H.-Q., Hu, J., Wang, D., Li, Z., Zhang, Q., Luo, Y., Yu, S.-H., & Jiang, H.-L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08773 · Cited by 1,166
Metal–organic frameworks as platforms for clean energy
Li, S.-L., & Xu, Q. (2013) · Energy & Environmental Science · doi:10.1039/c3ee40507a · Cited by 970
MOF positioning technology and device fabrication
Falcaro, P., Ricco, R., Doherty, C. M., Liang, K., Hill, A. J., & Styles, M. J. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00089g · Cited by 710
Photocatalytic Cr(VI) reduction in metal-organic frameworks: A mini-review
Wang, C.-C., Du, X.-D., Li, J., Guo, X.-X., Wang, P., & Zhang, J. (2016) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2016.04.030 · Cited by 659
Metadata
- Authors
- Gomes Silva, C., Luz, I., Llabrés i Xamena, F. X., Corma, A., & García, H.
- Venue
- Chemistry – A European Journal
- Publisher
- Wiley
- Published
- 2010-08-04
- Volume
- 16
- Issue
- 36
- Pages
- 11133-11138
- ISSN
- 0947-6539 (ISSN-L)
- 1521-3765
- OpenAlex
- W2157206861
- Cited by
- 866
- References
- 2
- FWCI
- 14.95
- Type
- journal article
- Language
- en
- Open access
- closed
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- Gomes Silva, C., Luz, I., Llabrés i Xamena, F. X., Corma, A., & García, H. (2010). Water Stable Zr–Benzenedicarboxylate Metal–Organic Frameworks as Photocatalysts for Hydrogen Generation. Chemistry – A European Journal. https://doi.org/10.1002/chem.200903526
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