The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Metal–Organic Frameworks as Efficient Heterogeneous Catalysts for the Regioselective Ring Opening of Epoxides
Abstract
An iron‐based metal–organic framework, [Fe(BTC)] (BTC: 1,3,5‐benzenetricarboxylate) is an efficient catalyst in the ring opening of styrene oxide with alcohols and aniline under mild reaction conditions. Out of the various alcohols tested for ring opening of styrene oxide, methanol was found to be the most reactive in terms of percentage conversion and reactivity. The rate of the ring‐opening reaction of styrene oxide decreases as the size of the alcohol is increased, suggesting the location of active sites in micropores. [Fe(BTC)] was a truly heterogeneous catalyst and could be reused without loss of activity. The analogous compound [Cu 3(BTC)2] was also found to be effective, although with somewhat lower activity than [Fe(BTC)]. The present heterogeneous protocol is compared with a homogeneous catalyst to give an insight into the reaction mechanism.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Cited by
Chen, Y.-Z., Zhou, Y.-X., Wang, H., Lu, J., Uchida, T., Xu, Q., Yu, S.-H., & Jiang, H.-L. (2015) · ACS Catalysis · doi:10.1021/cs501953d · Cited by 423
Metadata
- Authors
- Dhakshinamoorthy, A., Alvaro, M., & Garcia, H.
- Venue
- Chemistry – A European Journal
- Publisher
- Wiley
- Published
- 2010-07-19
- Volume
- 16
- Issue
- 28
- Pages
- 8530-8536
- ISSN
- 0947-6539 (ISSN-L)
- 1521-3765
- OpenAlex
- W2155337071
- Cited by
- 217
- References
- 1
- FWCI
- 12.04
- Type
- journal article
- Language
- en
- Open access
- closed
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- Dhakshinamoorthy, A., Alvaro, M., & Garcia, H. (2010). Metal–Organic Frameworks as Efficient Heterogeneous Catalysts for the Regioselective Ring Opening of Epoxides. Chemistry – A European Journal. https://doi.org/10.1002/chem.201000588
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