The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Size‐Dependent Structural Evolution and Chemical Reactivity of Gold Clusters
Abstract
Ground‐state structures and other experimentally relevant isomers of Au 15− to Au 24− clusters are determined through joint first‐principles density functional theory and photoelectron spectroscopy measurements. Subsequent calculations of molecular O 2 adsorption to the optimal cluster structures reveal a size‐dependent reactivity pattern that agrees well with earlier experiments. A detailed analysis of the underlying electronic structure shows that the chemical reactivity of the gold cluster anions can be elucidated in terms of a partial‐jellium picture, where delocalized electrons occupying electronic shells move over the ionic skeleton, whose geometric structure is strongly influenced by the directional bonding associated with the highly localized “d‐band” electrons.
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Citations
Cites
Charging Effects on Bonding and Catalyzed Oxidation of CO on Au 8 Clusters on MgO
Yoon, B., Häkkinen, H., Landman, U., Wörz, A. S., Antonietti, J.-M., Abbet, S., Judai, K., & Heiz, U. (2005) · Science · doi:10.1126/science.1104168 · Cited by 1,430
Self-citationBarnett, R. N., & Landman, U. (1993) · Physical Review B · doi:10.1103/physrevb.48.2081 · Cited by 629
Self-citation
Cited by
A unified view of ligand-protected gold clusters as superatom complexes
Walter, M., Akola, J., Lopez-Acevedo, O., Jadzinsky, P. D., Calero, G., Ackerson, C. J., Whetten, R. L., Grönbeck, H., & Häkkinen, H. (2008) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0801001105 · Cited by 1,742
Self-citationDensity functional theory for transition metals and transition metal chemistry
Cramer, C. J., & Truhlar, D. G. (2009) · Physical Chemistry Chemical Physics · doi:10.1039/b907148b · Cited by 1,648
Nonscalable Oxidation Catalysis of Gold Clusters
Yamazoe, S., Koyasu, K., & Tsukuda, T. (2014) · Accounts of Chemical Research · doi:10.1021/ar400209a · Cited by 607
Supracolloidal Reaction Kinetics of Janus Spheres
Chen, Q., Whitmer, J. K., Jiang, S., Bae, S. C., Luijten, E., & Granick, S. (2011) · Science · doi:10.1126/science.1197451 · Cited by 526
Metadata
- Authors
- Yoon, B., Koskinen, P., Huber, B., Kostko, O., von Issendorff, B., Häkkinen, H., Moseler, M., & Landman, U.
- Venue
- ChemPhysChem
- Publisher
- Wiley
- Published
- 2006-12-27
- Volume
- 8
- Issue
- 1
- Pages
- 157-161
- ISSN
- 1439-4235 (ISSN-L)
- 1439-7641
- OpenAlex
- W2129360151
- Cited by
- 210
- References
- 2
- FWCI
- 10.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yoon, B., Koskinen, P., Huber, B., Kostko, O., von Issendorff, B., Häkkinen, H., Moseler, M., & Landman, U. (2007). Size‐Dependent Structural Evolution and Chemical Reactivity of Gold Clusters. ChemPhysChem. https://doi.org/10.1002/cphc.200600524
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