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Determination of Band Structure Parameters and the Quasi‐Particle Gap of CdSe Quantum Dots by Cyclic Voltammetry
Abstract
Band structure parameters such as the conduction band edge, the valence band edge and the quasi‐particle gap of diffusing CdSe quantum dots (Q‐dots) of various sizes were determined using cyclic voltammetry. These parameters are strongly dependent on the size of the Q‐dots. The results obtained from voltammetric measurements are compared to spectroscopic and theoretical data. The fit obtained to the reported calculations based on the semi‐empirical pseudopotential method (SEPM)—especially in the strong size‐confinement region, is the best reported so far, according to our knowledge. For the smallest CdSe Q‐dots, the difference between the quasi‐particle gap and the optical band gap gives the electron–hole Coulombic interaction energy (Je1,h1). Interband states seen in the photoluminescence spectra were verified with cyclic voltammetry measurements.
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Citations
Cited by
Quantum Dots and Their Multimodal Applications: A Review
Bera, D., Qian, L., Tseng, T.-K., & Holloway, P. H. (2010) · Materials · doi:10.3390/ma3042260 · Cited by 1,365
Size-Dependent Valence and Conduction Band-Edge Energies of Semiconductor Nanocrystals
Jasieniak, J., Califano, M., & Watkins, S. E. (2011) · ACS Nano · doi:10.1021/nn201681s · Cited by 699
Metadata
- Authors
- Inamdar, S. N., Ingole, P. P., & Haram, S. K.
- Venue
- ChemPhysChem
- Publisher
- Wiley
- Published
- 2008-11-25
- Volume
- 9
- Issue
- 17
- Pages
- 2574-2579
- ISSN
- 1439-4235 (ISSN-L)
- 1439-7641
- OpenAlex
- W2136487485
- Cited by
- 228
- References
- 0
- FWCI
- 2.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Inamdar, S. N., Ingole, P. P., & Haram, S. K. (2008). Determination of Band Structure Parameters and the Quasi‐Particle Gap of CdSe Quantum Dots by Cyclic Voltammetry. ChemPhysChem. https://doi.org/10.1002/cphc.200800482
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