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Hydrogen Sulfide Adsorption on MOFs and MOF/Graphite Oxide Composites
Abstract
Composites of a copper‐based metal‐organic framework (MOF) and graphite oxide (GO) were tested for hydrogen sulfide removal at ambient conditions. In order to understand the mechanisms of adsorption, the initial and exhausted samples were analyzed by various techniques including X‐ray diffraction, Fourier transform infrared spectroscopy, thermogravimetric analyses, and sorption of nitrogen. Compared to the parent materials, an enhancement in hydrogen sulfide adsorption was found. It was the result of physical adsorption of water and H2S in the pore space formed at the interface between the MOF units and the graphene layers where the dispersive forces are the strongest. Besides physisorption, reactive adsorption was found as the main mechanism of retention. H2S molecules bind to the copper centers of the MOF. They progressively react with the MOF units resulting in the formation of copper sulfide. This leads to the collapse of the MOF structure. Water enhances adsorption in the composites as it allows the dissolution of hydrogen sulfide.
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Millward, A. R., & Yaghi, O. M. (2005) · Journal of the American Chemical Society · doi:10.1021/ja0570032 · Cited by 2,876
Cited by
Adsorptive desulfurization and denitrogenation using metal-organic frameworks
Ahmed, I., & Jhung, S. H. (2016) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2015.08.045 · Cited by 451
Composites of metal–organic frameworks: Preparation and application in adsorption
Ahmed, I., & Jhung, S. H. (2014) · Materials Today · doi:10.1016/j.mattod.2014.03.002 · Cited by 451
Kinetic stability of metal–organic frameworks for corrosive and coordinating gas capture
Rieth, A. J., Wright, A. M., & Dincă, M. (2019) · Nature Reviews Materials · doi:10.1038/s41578-019-0140-1 · Cited by 402
Stability of MOF-5 in a hydrogen gas environment containing fueling station impurities
Ming, Y., Purewal, J., Yang, J., Xu, C., Veenstra, M., Gaab, M., Müller, U., & Siegel, D. J. (2016) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2016.03.155 · Cited by 25
Metadata
- Authors
- Petit, C., Mendoza, B., & Bandosz, T. J.
- Venue
- ChemPhysChem
- Publisher
- Wiley
- Published
- 2010-10-13
- Volume
- 11
- Issue
- 17
- Pages
- 3678-3684
- ISSN
- 1439-4235 (ISSN-L)
- 1439-7641
- OpenAlex
- W2103348851
- Cited by
- 251
- References
- 1
- FWCI
- 15.82
- Type
- journal article
- Language
- en
- Open access
- closed
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- Petit, C., Mendoza, B., & Bandosz, T. J. (2010). Hydrogen Sulfide Adsorption on MOFs and MOF/Graphite Oxide Composites. ChemPhysChem. https://doi.org/10.1002/cphc.201000689
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