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Polariton Dynamics under Strong Light–Molecule Coupling
Abstract
We present a comprehensive experimental study of the photophysical properties of a molecule–cavity system under strong coupling conditions, using steady‐state and femtosecond time‐resolved emission and absorption techniques to selectively excite the lower and upper polaritons as well as the reservoir of uncoupled molecules. Our results demonstrate the complex decay routes in such hybrid systems and that, contrary to expectations, the lower polariton is intrinsically long‐lived.
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Citations
Cites
Room-Temperature Polariton Lasing in an Organic Single-Crystal Microcavity
Kéna-Cohen, S., & Forrest, S. R. (2010) · Nature Photonics · doi:10.1038/nphoton.2010.86 · Cited by 942
Cited by
Strong coupling between surface plasmon polaritons and emitters: a review
Törmä, P., & Barnes, W. L. (2015) · Reports on Progress in Physics · doi:10.1088/0034-4885/78/1/013901 · Cited by 1,644
Zengin, G., Wersäll, M., Nilsson, S., Antosiewicz, T. J., Käll, M., & Shegai, T. (2015) · Physical Review Letters · doi:10.1103/physrevlett.114.157401 · Cited by 566
Polaritonic Chemistry with Organic Molecules
Feist, J., Galego, J., & Garcia-Vidal, F. J. (2018) · ACS Photonics · doi:10.1021/acsphotonics.7b00680 · Cited by 438
Nonlinear optical signals and spectroscopy with quantum light
Dorfman, K. E., Schlawin, F., & Mukamel, S. (2016) · Reviews of Modern Physics · doi:10.1103/revmodphys.88.045008 · Cited by 361
Theoretical Advances in Polariton Chemistry and Molecular Cavity Quantum Electrodynamics
Mandal, A., Taylor, M. A. D., Weight, B. M., Koessler, E. R., Li, X., & Huo, P. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00855 · Cited by 270
Metadata
- Authors
- Schwartz, T., Hutchison, J. A., Léonard, J., Genet, C., Haacke, S., & Ebbesen, T. W.
- Venue
- ChemPhysChem
- Publisher
- Wiley
- Published
- 2012-12-11
- Volume
- 14
- Issue
- 1
- Pages
- 125-131
- ISSN
- 1439-4235 (ISSN-L)
- 1439-7641
- OpenAlex
- W2142920429
- Cited by
- 244
- References
- 1
- FWCI
- 4.98
- Type
- journal article
- Language
- en
- Open access
- closed
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- Schwartz, T., Hutchison, J. A., Léonard, J., Genet, C., Haacke, S., & Ebbesen, T. W. (2013). Polariton Dynamics under Strong Light–Molecule Coupling. ChemPhysChem. https://doi.org/10.1002/cphc.201200734
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