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Cleaving the βO4 Bonds of Lignin Model Compounds in an Acidic Ionic Liquid, 1‐H‐3‐Methylimidazolium Chloride: An Optional Strategy for the Degradation of Lignin
Abstract
The hydrolysis of βO4 bonds in two lignin model compounds was studied in an acidic ionic liquid, 1‐H‐3‐methylimidazolium chloride. The βO4 bonds of both guaiacylglycerol‐β‐guaiacyl ether and veratrylglycerol‐β‐guaiacyl ether underwent catalytic hydrolysis to produce guaiacol as the primary product with more than 70 % yield at 150 °C. Up to 32 wt % substrate concentration could be treated in the system without a decrease in guaiacol production. The ionic liquid could be reused without loss of activity in guaiacol production from both guaiacylglycerol‐β‐guaiacyl ether and veratrylglycerol‐β‐guaiacyl ether. A possible mechanism accounting for the guaiacol production is presented.
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The Catalytic Valorization of Lignin for the Production of Renewable Chemicals
Zakzeski, J., Bruijnincx, P. C. A., Jongerius, A. L., & Weckhuysen, B. M. (2010) · Chemical Reviews · doi:10.1021/cr900354u · Cited by 4,468
Metal Chlorides in Ionic Liquid Solvents Convert Sugars to 5-Hydroxymethylfurfural
Zhao, H., Holladay, J. E., Brown, H., & Zhang, Z. C. (2007) · Science · doi:10.1126/science.1141199 · Cited by 1,997
Self-citationReview of current and future softwood kraft lignin process chemistry
Chakar, F. S., & Ragauskas, A. J. (2004) · Industrial Crops and Products · doi:10.1016/j.indcrop.2004.04.016 · Cited by 1,203
Holladay, J. E., White, J. F., Bozell, J. J., & Johnson, D. (2007) · doi:10.2172/921839 · Cited by 905
Chemical aspects of kraft pulping
Gierer, J. (1980) · Wood Science and Technology · doi:10.1007/bf00383453 · Cited by 455
Cited by
Catalytic Transformation of Lignin for the Production of Chemicals and Fuels
Li, C., Zhao, X., Wang, A., Huber, G. W., & Zhang, T. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00155 · Cited by 2,951
Solid acid mediated hydrolysis of biomass for producing biofuels
Guo, F., Fang, Z., Xu, C. C., & Smith, R. L. (2012) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2012.04.001 · Cited by 276
Hong, S., Shen, X.-J., Pang, B., Xue, Z., Cao, X.-F., Wen, J.-L., Sun, Z.-H., Lam, S. S., Yuan, T.-Q., & Sun, R.-C. (2020) · Green Chemistry · doi:10.1039/d0gc00006j · Cited by 226
Pinkert, A., Goeke, D. F., Marsh, K. N., & Pang, S. (2011) · Green Chemistry · doi:10.1039/c1gc15671c · Cited by 199
Long, J., Lou, W., Wang, L., Yin, B., & Li, X. (2015) · Chemical Engineering Science · doi:10.1016/j.ces.2014.09.026 · Cited by 98
Diedericks, D., Rensburg, E. V., del Prado García‐Aparicio, M., & Görgens, J. F. (2012) · Biotechnology Progress · doi:10.1002/btpr.711 · Cited by 34
Metadata
- Authors
- Jia, S., Cox, B. J., Guo, X., Zhang, Z. C., & Ekerdt, J. G.
- Venue
- ChemSusChem
- Publisher
- Wiley
- Published
- 2010-07-30
- Volume
- 3
- Issue
- 9
- Pages
- 1078-1084
- ISSN
- 1864-5631 (ISSN-L)
- 1864-564X
- OpenAlex
- W2125007755
- Cited by
- 181
- References
- 5
- FWCI
- 4.19
- Type
- journal article
- Language
- en
- Open access
- closed
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