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Selective Hydrodeoxygenation of Biomass‐Derived Oxygenates to Unsaturated Hydrocarbons using Molybdenum Carbide Catalysts
Abstract
Which cleavage do you prefer? With a combination of density functional theory (DFT) calculations, surface science studies, and reactor evaluations, Mo(2)C is identified as a highly selective HDO catalyst to selectively convert biomass-derived oxygenates to unsaturated hydrocarbons through selective C-O bond scissions without C-C bond cleavage. This provides high-value HDO products for utilization as feedstocks for chemicals and fuels; this also reduces the overall consumption of H2 .
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Cited by
Bifunctional Catalysts for Upgrading of Biomass-Derived Oxygenates: A Review
Robinson, A. M., Hensley, J. E., & Medlin, J. W. (2016) · ACS Catalysis · doi:10.1021/acscatal.6b00923 · Cited by 548
Zhang, H., Wang, T., Wang, J., Liu, H., Dao, T. D., Li, M., Liu, G., Meng, X., Chang, K., Shi, L., et al. (2016) · Advanced Materials · doi:10.1002/adma.201505187 · Cited by 391
Molybdenum carbide as alternative catalyst for hydrogen production – A review
Ma, Y., Guan, G., Hao, X., Cao, J., & Abudula, A. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2016.11.092 · Cited by 294
Hydrotreatment of pyrolysis bio-oil: A review
Han, Y., Gholizadeh, M., Tran, C.-C., Kaliaguine, S., Li, C.-Z., Olarte, M., & Garcia-Perez, M. (2019) · Fuel Processing Technology · doi:10.1016/j.fuproc.2019.106140 · Cited by 292
Zhang, F., Wang, F., Wei, X., Yang, Y., Xu, S., Deng, D., & Wang, Y.-Z. (2022) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2021.12.052 · Cited by 269
Metadata
- Authors
- Ren, H., Yu, W., Salciccioli, M., Chen, Y., Huang, Y., Xiong, K., Vlachos, D. G., & Chen, J. G.
- Venue
- ChemSusChem
- Publisher
- Wiley
- Published
- 2013-04-04
- Volume
- 6
- Issue
- 5
- Pages
- 798-801
- ISSN
- 1864-5631 (ISSN-L)
- 1864-564X
- OpenAlex
- W2123201513
- Cited by
- 199
- References
- 0
- FWCI
- 11.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Ren, H., Yu, W., Salciccioli, M., Chen, Y., Huang, Y., Xiong, K., Vlachos, D. G., & Chen, J. G. (2013). Selective Hydrodeoxygenation of Biomass‐Derived Oxygenates to Unsaturated Hydrocarbons using Molybdenum Carbide Catalysts. ChemSusChem. https://doi.org/10.1002/cssc.201200991
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