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Nickel–Tungsten Carbide Catalysts for the Production of 2,5‐Dimethylfuran from Biomass‐Derived Molecules
Abstract
The development of new catalytic systems for the conversion of biomass‐derived molecules into liquid fuels has attracted much attention. We propose a non‐noble bimetallic catalyst based on nickel–tungsten carbide for the conversion of the platform molecules 5‐(hydroxymethyl)furfural into the liquid‐fuel molecule 2,5‐dimethylfuran (DMF). Different catalysts, metal ratios and reaction conditions have been tested and give rise to a 96% yield of DMF. The catalysts have been characterized and are discussed. The reaction mechanism is also explored through capture of reaction intermediates. The analysis of the reaction mixture over different catalysts is presented and helps to understand the role of nickel and tungsten carbide during the reaction.
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Citations
Cites
Chemical Routes for the Transformation of Biomass into Chemicals
Corma, A., Iborra, S., & Velty, A. (2007) · Chemical Reviews · doi:10.1021/cr050989d · Cited by 5,970
Metal Chlorides in Ionic Liquid Solvents Convert Sugars to 5-Hydroxymethylfurfural
Zhao, H., Holladay, J. E., Brown, H., & Zhang, Z. C. (2007) · Science · doi:10.1126/science.1141199 · Cited by 1,997
Cited by
Ni-based bimetallic heterogeneous catalysts for energy and environmental applications
De, S., Zhang, J., Luque, R., & Yan, N. (2016) · Energy & Environmental Science · doi:10.1039/c6ee02002j · Cited by 786
Hu, L., Lin, L., Wu, Z., Zhou, S., & Liu, S. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.02.042 · Cited by 445
De, S., Saha, B., & Luque, R. (2015) · Bioresource Technology · doi:10.1016/j.biortech.2014.09.065 · Cited by 359
Efficient valorization of biomass to biofuels with bifunctional solid catalytic materials
Li, H., Fang, Z., Smith, R. L., & Yang, S. (2016) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2016.04.004 · Cited by 284
Metadata
- Authors
- Huang, Y., Chen, M., Yan, L., Guo, Q., & Fu, Y.
- Venue
- ChemSusChem
- Publisher
- Wiley
- Published
- 2014-02-26
- Volume
- 7
- Issue
- 4
- Pages
- 1068-1072
- ISSN
- 1864-5631 (ISSN-L)
- 1864-564X
- OpenAlex
- W2072438113
- Cited by
- 199
- References
- 2
- FWCI
- 11.09
- Type
- journal article
- Language
- en
- Open access
- closed
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- Huang, Y., Chen, M., Yan, L., Guo, Q., & Fu, Y. (2014). Nickel–Tungsten Carbide Catalysts for the Production of 2,5‐Dimethylfuran from Biomass‐Derived Molecules. ChemSusChem. https://doi.org/10.1002/cssc.201301356
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