The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Hydrogen‐free catalytic fractionation of woody biomass
Open accessAbstract
The pulping industry could become a biorefinery if the lignin and hemicellulose components of the lignocellulose are valorized. Conversion of lignin into well‐defined aromatic chemicals is still a major challenge. Lignin depolymerization reactions often occur in parallel with irreversible condensation reactions of the formed fragments. Here, we describe a strategy that markedly suppresses the undesired condensation pathways and allows to selectively transform lignin into a few aromatic compounds. Notably, applying this strategy to woody biomass at organosolv pulping conditions, the hemicellulose, cellulose, and lignin were separated and in parallel the lignin was transformed into aromatic monomers. In addition, we were able to utilize a part of the lignocellulose as an internal source of hydrogen for the reductive lignin transformations. We hope that the presented methodology will inspire researchers in the field of lignin valorization as well as pulp producers to develop more efficient biomass fractionation processes in the future.
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Cites
Chemical Routes for the Transformation of Biomass into Chemicals
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The Catalytic Valorization of Lignin for the Production of Renewable Chemicals
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Catalytic Transformation of Lignin for the Production of Chemicals and Fuels
Li, C., Zhao, X., Wang, A., Huber, G. W., & Zhang, T. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00155 · Cited by 2,951
Lignin depolymerisation strategies: towards valuable chemicals and fuels
Xu, C., Arancon, R. A. D., Labidi, J., & Luque, R. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00235k · Cited by 1,031
Cited by
Chemicals from lignin: an interplay of lignocellulose fractionation, depolymerisation, and upgrading
Schutyser, W., Renders, T., Van den Bosch, S., Koelewijn, S.-F., Beckham, G. T., & Sels, B. F. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00566k · Cited by 2,552
Lignin-first biomass fractionation: the advent of active stabilisation strategies
Renders, T., Van den Bosch, S., Koelewijn, S.-F., Schutyser, W., & Sels, B. F. (2017) · Energy & Environmental Science · doi:10.1039/c7ee01298e · Cited by 709
Lignin valorization: Status, challenges and opportunities
Sethupathy, S., Murillo Morales, G., Gao, L., Wang, H., Yang, B., Jiang, J., Sun, J., & Zhu, D. (2022) · Bioresource Technology · doi:10.1016/j.biortech.2022.126696 · Cited by 473
Reductive catalytic fractionation: state of the art of the lignin-first biorefinery
Renders, T., Van den Bossche, G., Vangeel, T., Van Aelst, K., & Sels, B. (2019) · Current Opinion in Biotechnology · doi:10.1016/j.copbio.2018.12.005 · Cited by 437
Van den Bosch, S., Renders, T., Kennis, S., Koelewijn, S.-F., Van den Bossche, G., Vangeel, T., Deneyer, A., Depuydt, D., Courtin, C. M., Thevelein, J. M., et al. (2017) · Green Chemistry · doi:10.1039/c7gc01324h · Cited by 346
Biomass Fractionation and Lignin Fractionation towards Lignin Valorization
Xu, J., Li, C., Dai, L., Xu, C., Zhong, Y., Yu, F., & Si, C. (2020) · ChemSusChem · doi:10.1002/cssc.202001491 · Cited by 317
Flowthrough Reductive Catalytic Fractionation of Biomass
Anderson, E. M., Stone, M. L., Katahira, R., Reed, M., Beckham, G. T., & Román-Leshkov, Y. (2017) · Joule · doi:10.1016/j.joule.2017.10.004 · Cited by 288
Liu, X., Bouxin, F. P., Fan, J., Budarin, V. L., Hu, C., & Clark, J. H. (2021) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2020.123490 · Cited by 71
Degradation of vanillin during lignin valorization under alkaline oxidation
Zhu, Y., Liu, J., Liao, Y., Lv, W., Ma, L., & Wang, C. (2018) · Topics in Current Chemistry · doi:10.1007/s41061-018-0208-1 · Cited by 46
Qiu, S., Wang, M., Fang, Y., & Tan, T. (2020) · Sustainable Energy & Fuels · doi:10.1039/d0se01118e · Cited by 39
Economical concerns of lignin in the energy sector
Sharma, A., Kaur, P., Singh, G., & Arya, S. K. (2021) · Cleaner Engineering and Technology · doi:10.1016/j.clet.2021.100258 · Cited by 38
Metadata
- Authors
- Galkin, M. V., Smit, A. T., Subbotina, E., Artemenko, K. A., Bergquist, J., Huijgen, W. J. J., & Samec, J. S. M.
- Venue
- ChemSusChem
- Publisher
- Wiley
- Published
- 2016-11-15
- Volume
- 9
- Issue
- 23
- Pages
- 3280-3287
- ISSN
- 1864-5631 (ISSN-L)
- 1864-564X
- OpenAlex
- W2553940241
- Cited by
- 192
- References
- 4
- FWCI
- 8.06
- Type
- journal article
- Language
- en
- Open access
- green
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