Process intensification routes for mineral carbonation*
Open accessAbstract
Abstract Mineral carbonation is a realistic route for capture and storage of carbon dioxide. The principal advantages of this approach are the chemical stability and storage safety of mineral carbonates, the opportunities for process integration available, and the potential for conversion of low‐value materials into useful products. In this work, the valorization of alkaline waste materials from thermal processes by mineral carbonation utilizing intensified and integrated mineral carbonation routes is explored. Process intensification aims at providing the paradigm‐shifting techniques needed to revolutionize the chemical engineering industry in the twenty‐first century, particularly focusing on improvements toward process efficiency, yield, and sustainability. The combination of process intensification and process integration strategies has the potential to produce economically feasible and industrially acceptable carbonation technologies that can soon be implemented large scale, several examples of which are already proven at laboratory scale and are herein discussed. © 2011 Society of Chemical Industry and John Wiley & Sons, Ltd
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The particle size is a key parameter affecting carbonation because reducing size increases surface area and consequently the availability of reactive Mg and Ca.
“The particle size is a key parameter affecting carbonation because the reduction of size increases surface area and consequently the availability of reactive Mg and Ca.65”
From A review of mineral carbonation technologies to sequester CO <sub>2</sub> (2014) · cites this paper as [65]
The liquid/solid (L/S) ratio is an important parameter because carbonation requires specific L/S ratios to be efficient.
“The liquid/solid (L/S) ratio is an important parameter because carbonation requires specific L/S ratios to be efficient.65”
From A review of mineral carbonation technologies to sequester CO <sub>2</sub> (2014) · cites this paper as [65]
Temperature influences both the dissolution of CO2 in water (dissolution decreases with temperature) and dissolution of calcium and magnesium from minerals (dissolution increases when temperature increases).
“Temperature influences both the dissolution of CO 2 in water (dissolution decreases with temperature) and dissolution of calcium and magnesium from the minerals (dissolution increases when temperature increases).”
From A review of mineral carbonation technologies to sequester CO <sub>2</sub> (2014) · cites this paper as [65]
Low temperatures enhance the diffusion of CO2 in the carbonated shell, while high temperatures increase the magnesium and calcium available.
“Low temperatures enhance the diffusion of CO 2 in the carbonated shell, while high temperatures increase the magnesium and calcium available.65,67”
From A review of mineral carbonation technologies to sequester CO <sub>2</sub> (2014) · cites this paper as [65]
Stirring or sonication during carbonation limits the formation of carbonate shells, allowing further dissolution of Mg and Ca and diffusion of CO2.
“Stirring or sonication during carbonation limits the formation of carbonate shells, allowing further dissolution of Mg and Ca and diffusion of CO 2 .65”
From A review of mineral carbonation technologies to sequester CO <sub>2</sub> (2014) · cites this paper as [65]
Cites
CO2 capture and separation technologies for end-of-pipe applications – A review
Olajire, A. A. (2010) · Energy · doi:10.1016/j.energy.2010.02.030 · Cited by 1,217 · see citing works
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A review of mineral carbonation technologies to sequester CO <sub>2</sub>
Sanna, A., Uibu, M., Caramanna, G., Kuusik, R., & Maroto-Valer, M. M. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00035h · Cited by 1,194 · see citing works
A review of mineral carbonation technology in sequestration of CO2
Olajire, A. A. (2013) · Journal of Petroleum Science and Engineering · doi:10.1016/j.petrol.2013.03.013 · Cited by 567 · see citing works
Santos, R. M., Van Bouwel, J., Vandevelde, E., Mertens, G., Elsen, J., & Van Gerven, T. (2013) · International Journal of Greenhouse Gas Control · doi:10.1016/j.ijggc.2013.04.004 · Cited by 257 · see citing works
Self-citationWaste materials for carbon capture and storage by mineralisation (CCSM)–A UK perspective
Sanna, A., Dri, M., Hall, M. R., & Maroto-Valer, M. (2012) · Applied Energy · doi:10.1016/j.apenergy.2012.06.049 · Cited by 159 · see citing works
Ultrasound-intensified mineral carbonation
Santos, R. M., François, D., Mertens, G., Elsen, J., & Van Gerven, T. (2013) · Applied Thermal Engineering · doi:10.1016/j.applthermaleng.2012.03.035 · Cited by 141 · see citing works
Self-citationChiang, Y. W., Santos, R. M., Monballiu, A., Ghyselbrecht, K., Martens, J. A., Mattos, M. L. T., Gerven, T. V., & Meesschaert, B. (2013) · Minerals Engineering · doi:10.1016/j.mineng.2012.09.004 · Cited by 44 · see citing works
Self-citation
- Authors
- Santos, R. M., & Van Gerven, T.
- Affiliations
- KU Leuven (BE)
- ORCID
- Santos, Rafael M.
- Venue
- Greenhouse Gases: Science and Technology
- Publisher
- Wiley
- Published
- 2011-09-30
- Volume
- 1
- Issue
- 4
- Pages
- 287-293
- ISSN
- 2152-3878 (ISSN-L)
- OpenAlex
- W2060090224
- Cited by
- 39
- References
- 1
- Citations by year
- 2026: 2 · 2024: 2 · 2023: 3 · 2022: 1 · 2021: 3 · 2020: 4 · 2018: 1 · 2016: 6 · 2014: 3 · 2013: 7 · 2012: 5
- FWCI
- 4.83
- Type
- journal article
- Language
- en
- Open access
- green
- lirias.kuleuven.be
- Licence
- Locations
- Greenhouse Gases Science and Technology (publishedVersion)
- Lirias (KU Leuven) (submittedVersion, other-oa)
- Funders
- Natural Sciences and Engineering Research Council of Canada
- Topics
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
- Keywords
- CO2 mineralization, process intensification, process integration, carbon capture and storage, waste valorization, carbonate minerals, carbon sequestration
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