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Cited by 32High-Temperature Coating BehaviorsMetallurgical Processes and ThermodynamicsIron oxide chemistry and applications

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Oxidation of iron at 600 °C – experiments and simulations

Larsson, H., Jonsson, T., Naraghi, R., Gong, Y., Reed, R. C., Ågren, J.·2017·Materials and Corrosion
DOI 10.1002/maco.201508781
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Abstract

Pure iron has been oxidized at 600 °C and 1 bar in dry O 2 (oxygen partial pressure 0.05, bal. N 2) and the mass gain as well as the thicknesses of the individual oxide phases have been measured. The oxidation process has been simulated using a modified version of the homogenization model as implemented in Dictra; this has helped to rationalize the kinetics of oxide scale formation and in particular the evolution of the hematite (Fe 2 O 3), magnetite (Fe 3 O 4), and wustite (FeO) which form. Independently assessed thermodynamic and kinetic Calphad databases are needed for the calculations; details of these are given. Reasonable agreement between simulation results and experimental data is obtained, though it is concluded that the large influence of grain boundary diffusion on the oxidation rate needs further consideration.

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Metadata

Authors
Larsson, H., Jonsson, T., Naraghi, R., Gong, Y., Reed, R. C., & Ågren, J.
Affiliations
  • KTH Royal Institute of Technology (SE)
  • Chalmers University of Technology (SE)
  • Thermo‐Calc Software Norra Stationsgatan 93 SE‐11364 Stockholm Sweden
  • University of Oxford (GB)
Corresponding author
Larsson, H.
ORCID
Venue
Materials and Corrosion
Publisher
Wiley
Published
2016-04-21
Volume
68
Issue
2
Pages
133-142
ISSN
  • 0043-2822 (ISSN-L)
  • 0947-5117
  • 1521-4176
DOI
10.1002/maco.201508781
OpenAlex
W2340229924
Cited by
32
References
0
Citations by year
2026: 2 · 2025: 4 · 2024: 2 · 2023: 4 · 2021: 7 · 2020: 8 · 2018: 4 · 2017: 1
FWCI
2.04
Type
journal article
Language
en
Open access
closed
Licence
onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations
  • Materials and Corrosion (publishedVersion)
  • Chalmers Publication Library (Chalmers University of Technology) (submittedVersion)
  • Chalmers Research (Chalmers University of Technology) (submittedVersion)
Funders
VINNOVA
Topics
  • Physical Sciences › Materials Science › Surfaces, Coatings and Films › High-Temperature Coating Behaviors
  • Physical Sciences › Materials Science › Metals and Alloys › Metallurgical Processes and Thermodynamics
  • Physical Sciences › Materials Science › Materials Chemistry › Iron oxide chemistry and applications
Keywords
iron oxidation, high-temperature oxidation, oxide scale formation, hematite, magnetite, wüstite, oxide scale thickness, mass gain, homogenization model, oxidation kinetics, grain boundary diffusion, CALPHAD thermodynamic database, DICTRA

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