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Novel Hyperbranched Poly([1,2,3]‐triazole)s Derived from AB2 Monomers by a 1,3‐Dipolar Cycloaddition
Abstract
Summary: Novel hyperbranched poly([1,2,3]‐triazole)s were synthesized from several AB 2 monomers by a 1,3‐dipolar cycloaddition reaction. The compound 3,5‐bis(propargyloxy)benzyl azide was polymerized thermally at room temperature leading to 1,4‐ and 1,5‐disubstituted poly([1,2,3]‐triazole) and catalytically leading only to the 1,4‐disubstituted poly([1,2,3]‐triazole). Only the thermal reaction led to fully soluble products. The AB 2 monomers containing an internal alkyne A unit could be autopolymerized thermally under mild reaction conditions leading to soluble, high‐molecular‐weight hyperbranched poly([1,2,3] triazole)s. All products were characterized by detailed NMR investigations. Synthesis route for polymers 8a and 8b. imageSynthesis route for polymers 8a and 8b.
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Cited by
CuI‐Catalyzed Alkyne–Azide “Click” Cycloadditions from a Mechanistic and Synthetic Perspective
Bock, V. D., Hiemstra, H., & van Maarseveen, J. H. (2006) · European Journal of Organic Chemistry · doi:10.1002/ejoc.200500483 · Cited by 1,452
Marrying click chemistry with polymerization: expanding the scope of polymeric materials
Golas, P. L., & Matyjaszewski, K. (2010) · Chem. Soc. Rev. · doi:10.1039/b901978m · Cited by 863
Qin, A., Lam, J. W. Y., & Tang, B. Z. (2010) · Chemical Society Reviews · doi:10.1039/b909064a · Cited by 587
“Click”‐Chemistry in Polymer and Material Science: the Update
Binder, W. H. (2008) · Macromolecular Rapid Communications · doi:10.1002/marc.200800332 · Cited by 567
Metadata
- Authors
- Scheel, A. J., Komber, H., & Voit, B. I.
- Venue
- Macromolecular Rapid Communications
- Publisher
- Wiley
- Published
- 2004-06
- Volume
- 25
- Issue
- 12
- Pages
- 1175-1180
- ISSN
- 1022-1336 (ISSN-L)
- 1521-3927
- OpenAlex
- W2161671106
- Cited by
- 169
- References
- 0
- FWCI
- 8.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Scheel, A. J., Komber, H., & Voit, B. I. (2004). Novel Hyperbranched Poly([1,2,3]‐triazole)s Derived from AB2 Monomers by a 1,3‐Dipolar Cycloaddition. Macromolecular Rapid Communications. https://doi.org/10.1002/marc.200400097
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