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Introduction to living polymeriz. Living and/or controlled polymerization
Abstract
The effects of various imperfections such as slow initiation, termination, transfer and slow exchange on kinetics, molecular weights and polydispersities in chain growth polymerizations are simulated. The simukations demonstrate that well defined polymers polymers can be prepared in systems with chain‐breaking reactions. Thus, under carefully selected conditions, non‐living polyumerizations may provide controlled polymers. On the other hand, polymers with unpredictable molecular weights and broad and even polymodal molecular weight distributions can be formed in living systems without irreversible transfer and termination. In some living systems molecular weights may stay constant or even decrease with conversion. Therefore, a clear distrinction should be made between living and polymerizations.
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Citations
Cites
SZWARC, M. (1956) · Nature · doi:10.1038/1781168a0 · Cited by 1,360
Cited by
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Meier, M. A. R., Metzger, J. O., & Schubert, U. S. (2007) · Chemical Society Reviews · doi:10.1039/b703294c · Cited by 1,487
Matyjaszewski, K., Patten, T. E., & Xia, J. (1997) · Journal of the American Chemical Society · doi:10.1021/ja963361g · Cited by 891
Self-citationMarrying click chemistry with polymerization: expanding the scope of polymeric materials
Golas, P. L., & Matyjaszewski, K. (2010) · Chem. Soc. Rev. · doi:10.1039/b901978m · Cited by 863
Self-citationControlled/living radical polymerization in aqueous media: homogeneous and heterogeneous systems
Qiu, J., Charleux, B., & Matyjaszewski, K. (2001) · Progress in Polymer Science · doi:10.1016/s0079-6700(01)00033-8 · Cited by 595
Self-citationVisible Light and Sunlight Photoinduced ATRP with ppm of Cu Catalyst
Konkolewicz, D., Schröder, K., Buback, J., Bernhard, S., & Matyjaszewski, K. (2012) · ACS Macro Letters · doi:10.1021/mz300457e · Cited by 593
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Metadata
- Authors
- Matyjaszewski, K.
- Venue
- Journal of Physical Organic Chemistry
- Publisher
- Wiley
- Published
- 1995-04
- Volume
- 8
- Issue
- 4
- Pages
- 197-207
- ISSN
- 0894-3230 (ISSN-L)
- 1099-1395
- OpenAlex
- W1999404445
- Cited by
- 170
- References
- 1
- FWCI
- 6.04
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
