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Gamma‐, photo‐, and thermally‐initiated oxidation of linear low density polyethylene: A quantitative comparison of oxidation products
Abstract
The detailed oxidation products from the initiated oxidation of linear low density polyethylene have been compared by the use of infrared spectroscopy combined with chemical derivatization. Oxidized films were treated with NO or SF 4 to allow the resolution of the various alcohol and hydroperoxides and of the carbonyl species, respectively. All types of initiation gave very similar products but in varying quantities. In photooxidation, hydroperoxide was clearly shown to approach a photostationary concentration either from below for fresh film or from above for samples that had been pre‐oxidized by γ‐irradiation, prior to UV exposure. Carboxylic acid groups, the main backbone scission product, dominated in photooxidations, possibly as the result of the further oxidation of sec‐hydroperoxide sites.
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Citations
Cited by
Brandon, J., Goldstein, M., & Ohman, M. D. (2016) · Marine Pollution Bulletin · doi:10.1016/j.marpolbul.2016.06.048 · Cited by 626
Gardette, M., Perthue, A., Gardette, J.-L., Janecska, T., Földes, E., Pukánszky, B., & Therias, S. (2013) · Polymer Degradation and Stability · doi:10.1016/j.polymdegradstab.2013.07.017 · Cited by 566
Post electron-beam irradiation oxidation of orthopaedic UHMWPE
Costa, L., Carpentieri, I., & Bracco, P. (2008) · Polymer Degradation and Stability · doi:10.1016/j.polymdegradstab.2008.06.003 · Cited by 78
Ultra-high molecular weight polyethylene: I. Mechano-oxidative degradation
Costa, L., Luda, M. P., & Trossarelli, L. (1997) · Polymer Degradation and Stability · doi:10.1016/s0141-3910(96)00170-x · Cited by 66
Metadata
- Authors
- Lacoste, J., & Carlsson, D. J.
- Venue
- Journal of Polymer Science Part A: Polymer Chemistry
- Publisher
- Wiley
- Published
- 1992-03-15
- Volume
- 30
- Issue
- 3
- Pages
- 493-500
- ISSN
- 0887-624X (ISSN-L)
- 1099-0518
- OpenAlex
- W2134404503
- Cited by
- 283
- References
- 0
- FWCI
- 11.64
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Gamma‐, photo‐, and thermally‐initiated oxidation of linear low density polyethylene: A quantitative comparison of oxidation products. https://app.cochat.ai/papers/10.1002/pola.1992.080300316
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- Lacoste, J., & Carlsson, D. J. (1992). Gamma‐, photo‐, and thermally‐initiated oxidation of linear low density polyethylene: A quantitative comparison of oxidation products. Journal of Polymer Science Part A: Polymer Chemistry. https://doi.org/10.1002/pola.1992.080300316
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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