Paving the way for solution‐ processable perovskite lasers
Abstract
Trihalide perovskites have been studied quite extensively as light‐harvesting media in photovoltaic devices and have shown a peculiar blend of optoelectronic properties, particularly remarkable carrier mobilities, diffusion lengths comparable to those of inorganic semiconductors and band gap tuneability. Only limited research effort, though, has been devoted so far to leveraging such properties for light emission, and many related processes remain unclear. Here, we identify organic‐inorganic metal halide perovskites as promising candidates for replacing a variety of raw materials at risk of supply shortage, currently used in manufacturing gain media for commercial lasers. We investigate the dynamics of light emission by transient photoluminescence spectroscopy and on the grounds of our findings we identify the challenges ahead on the way to engineering perovskite‐based lasers. (© 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
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Amplified spontaneous emission (ASE) has been observed via optical pumping of perovskite thin films even with pulses longer than 100 ns.
“With amplified spontaneous emission (ASE) observed via optical pumping of perovskite thin films even with pulses longer than 100 ns [11], these devices show a great promise for continuous wave lasing.”
From Integrated perovskite lasers on a silicon nitride waveguide platform by cost-effective high throughput fabrication (2017) · cites this paper as [11]
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Cegielski, P. J., Neutzner, S., Porschatis, C., Lerch, H., Bolten, J., Suckow, S., Kandada, A. R. S., Chmielak, B., Petrozza, A., Wahlbrink, T., et al. (2017) · Optics Express · doi:10.1364/oe.25.013199 · Cited by 67 · see citing works
- Authors
- Sarritzu, V., Cadelano, M., Sestu, N., Marongiu, D., Piras, R., Chang, X., Quochi, F., Saba, M., Mura, A., & Bongiovanni, G.
- Affiliations
- University of Cagliari (IT)
- Corresponding author
- Sarritzu, Valerio
- ORCID
- Venue
- physica status solidi c
- Publisher
- Wiley
- Published
- 2016-09-21
- Volume
- 13
- Issue
- 10-12
- Pages
- 1028-1033
- ISSN
- 1610-1634 (ISSN-L)
- 1862-6351
- 1610-1642
- OpenAlex
- W2525662948
- Cited by
- 3
- References
- 0
- Citations by year
- 2022: 1 · 2019: 2
- FWCI
- 0.31
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Physica status solidi. C, Conferences and critical reviews/Physica status solidi. C, Current topics in solid state physics (publishedVersion)
- UNICA IRIS Institutional Research Information System (University of Cagliari) (submittedVersion)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Perovskite Materials and Applications
- Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
- Physical Sciences › Materials Science › Materials Chemistry › Luminescence Properties of Advanced Materials
- Keywords
- perovskite lasers, organic-inorganic hybrid perovskites, solution processing, transient photoluminescence, gain medium, carrier mobility, light-harvesting materials
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