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Bioinspired Patterning with Extreme Wettability Contrast on TiO2 Nanotube Array Surface: A Versatile Platform for Biomedical Applications
Abstract
Binary wettability patterned surfaces with extremely high wetting contrasts can be found in nature on living creatures. They offer a versatile platform for microfluidic management. In this work, a facile approach to fabricating erasable and rewritable surface patterns with extreme wettability contrasts (superhydrophilic/superhydrophobic) on a TiO 2 nanotube array (TNA) surface through self‐assembly and photocatalytic lithography is reported. The multifunctional micropatterned superhydrophobic TNA surface can act as a 2D scaffold for site‐selective cell immobilization and reversible protein absorption. Most importantly, such a high‐contrast wettability template can be used to construct various well‐defined 3D functional patterns, such as calcium phosphate, silver nanoparticles, drugs, and biomolecules in a highly selective manner. The 3D functional patterns would be a versatile platform in a wide range of applications, especial for biomedical devices (e.g., high‐throughput molecular sensing, targeted antibacterials, and drug delivery). In a proof‐of‐concept study, the surface‐enhanced Raman scattering and antibacterial performance of the fabricated 3D AgNP@TNA pattern, and the targeted drug delivery for site‐specific and high‐sensitivity cancer cell assays was investigated.
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Wettability of porous surfaces
Cassie, A. B. D., & Baxter, S. (1944) · Transactions of the Faraday Society · doi:10.1039/tf9444000546 · Cited by 13,807
Cited by
Recent advances in the potential applications of bioinspired superhydrophobic materials
Darmanin, T., & Guittard, F. (2014) · J. Mater. Chem. A · doi:10.1039/c4ta02071e · Cited by 555
One‐dimensional TiO2 Nanotube Photocatalysts for Solar Water Splitting
Ge, M., Li, Q., Cao, C., Huang, J., Li, S., Zhang, S., Chen, Z., Zhang, K., Al‐Deyab, S. S., & Lai, Y. (2017) · Advanced Science · doi:10.1002/advs.201600152 · Cited by 555
Self-citationWang, B., Xu, Q., Ye, Z., Liu, H., Lin, Q., Nan, K., Li, Y., Wang, Y., Qi, L., & Chen, H. (2016) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.6b08893 · Cited by 130
Metadata
- Authors
- Lai, Y., Lin, L., Pan, F., Huang, J., Song, R., Huang, Y., Lin, C., Fuchs, H., & Chi, L.
- Venue
- Small
- Publisher
- Wiley
- Published
- 2013-02-18
- Volume
- 9
- Issue
- 17
- Pages
- 2945-2953
- ISSN
- 1613-6810 (ISSN-L)
- 1613-6829
- OpenAlex
- W1998034768
- Cited by
- 171
- References
- 1
- FWCI
- 8.41
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lai, Y., Lin, L., Pan, F., Huang, J., Song, R., Huang, Y., Lin, C., Fuchs, H., & Chi, L. (2013). Bioinspired Patterning with Extreme Wettability Contrast on TiO2 Nanotube Array Surface: A Versatile Platform for Biomedical Applications. Small. https://doi.org/10.1002/smll.201300187
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