Topology optimisation of biphasic adsorbent beds for gas storage
Open accessAbstract
Adsorption is a retention mechanism of fluid molecules on solid surfaces and presents a wide range of applications, such as fuel storage, refrigeration and separation processes. This work describes the modelling of gas adsorption on porous media and presents an optimisation approach for the design of adsorption systems based on biphasic adsorbent beds by topology optimisation. A comprehensive formulation for the adsorption phenomenon is presented, detailing the derivation of governing equations and respective weak forms and discretisation for the implementation of the finite element method (FEM). A new topology optimisation material model based on offset hyperbolic tangents is introduced. The derivation of sensitivities is presented in detail, based on a transient adjoint problem. A diverse set of optimised adsorbed natural gas (ANG) tanks, considering real material properties of activated carbon and steel, is presented. Results indicate the suitability of the method in optimising the distribution of phases across adsorbent beds and show that biphasic ANG tanks can perform significantly better than traditional tanks.
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Application of topology optimization to adsorption systems specifically is scarce.
“Its application to adsorption systems specifically, however, is quite scarce.”
From Topology optimisation of adsorption beds for cost-effective direct air capture (2026) · cites this paper as [23]
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Cited by
Sorted by citations
Topology optimisation of adsorption beds for cost-effective direct air capture
Mallon, C., Thornton, A., Hill, M., Badia, S., & Grutering, N. (2026) · arXiv · doi:10.48550/arxiv.2609.14214
“In [23] and [24], optimizations considering adsorption in natural gas storage systems are conducted.”
- Authors
- Amigo, R. C. R., Prado, D. S., Paiva, J. L., Hewson, R. W., & Silva, E. C. N.
- Affiliations
- Universidade de São Paulo (BR)
- Imperial College London (GB)
- Corresponding author
- Amigo, R. C. R.
- Venue
- Structural and Multidisciplinary Optimization
- Published
- 2018-10-27
- Volume
- 58
- Issue
- 6
- Pages
- 2431-2454
- ISSN
- 1615-147X (ISSN-L)
- 1615-1488
- OpenAlex
- W2898372437
- Cited by
- 13
- References
- 0
- Citations by year
- 2026: 4 · 2025: 2 · 2023: 1 · 2022: 1 · 2021: 4 · 2020: 1
- FWCI
- 1.12
- Type
- journal article
- Language
- en
- Open access
- hybrid
- doi.org
- Licence
- Locations
- Structural and Multidisciplinary Optimization (publishedVersion, cc-by)
- Spiral (Imperial College London) (submittedVersion, cc-by)
- Funders
- Conselho Nacional de Desenvolvimento Científico e Tecnológico (200404/2014-8)
- Fundação de Amparo à Pesquisa do Estado de São Paulo (2014/50279-4)
- Topics
- Physical Sciences › Engineering › Civil and Structural Engineering › Topology Optimization in Engineering
- Physical Sciences › Engineering › Mechanical Engineering › Cellular and Composite Structures
- Physical Sciences › Engineering › Computational Mechanics › Advanced Numerical Methods in Computational Mathematics
- Keywords
- topology optimization, gas adsorption, adsorbed natural gas, gas storage tanks, porous media, activated carbon, sensitivity analysis, phase distribution, finite element formulation
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