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Modeling ionic strength effects on anion adsorption at hydrous oxide/solution interfaces
Open accessAbstract
The effects of changes in ionic strength on the adsorption behavior of selenite (SeO32−) and selenate (SeO42−) on goethite and hydrous ferric oxide have been modeled using a generalized version of the triple-layer surface complexation model. Selenite adsorption, which is relatively unaffected by changes in ionic strength, is best modeled assuming that selenite forms an inner-sphere (surface coordination) complex; selenate adsorption, which is markedly reduced by increasing ionic strength, is best modeled assuming that selenate forms an outer-sphere (ion-pair) surface complex. The modeling results suggest that it is possible to distinguish between inner-sphere and outer-sphere anion surface complexes by studying the effects of ionic strength on anion partitioning.
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Cited by
Zhu, X., Li, B., Yang, J., Li, Y., Zhao, W., Shi, J., & Gu, J. (2015) · ACS Applied Materials & Interfaces · doi:10.1021/am5059074 · Cited by 486
Selenium environmental cycling and bioavailability: A structural chemist point of view
Fernández-Martínez, A., & Charlet, L. (2009) · Reviews in Environmental Science and Bio/Technology · doi:10.1007/s11157-009-9145-3 · Cited by 487
Adsorption and Polymerization of Amino Acids on Mineral Surfaces: A Review
Lambert, J.-F. (2008) · Origins of Life and Evolution of Biospheres · doi:10.1007/s11084-008-9128-3 · Cited by 443
Goh, K.-H., & Lim, T.-T. (2004) · Chemosphere · doi:10.1016/j.chemosphere.2003.11.041 · Cited by 305
Selenate and Selenite Sorption on Iron Oxides An Infrared and Electrophoretic Study
Su, C., & Suarez, D. L. (2000) · Soil Science Society of America Journal · doi:10.2136/sssaj2000.641101x · Cited by 261
Metadata
- Authors
- Hayes, K. F., Papelis, C., & Leckie, J. O.
- Venue
- Journal of Colloid and Interface Science
- Publisher
- Elsevier BV
- Published
- 1988-10
- Volume
- 125
- Issue
- 2
- Pages
- 717-726
- ISSN
- 0021-9797 (ISSN-L)
- OpenAlex
- W4231922294
- Cited by
- 471
- References
- 0
- FWCI
- 5.49
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Hayes, K. F., Papelis, C., & Leckie, J. O. (1988). Modeling ionic strength effects on anion adsorption at hydrous oxide/solution interfaces. Journal of Colloid and Interface Science. https://doi.org/10.1016/0021-9797(88)90039-2
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