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Cited by 614

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Regime III crystallization in melt-crystallized polymers: The variable cluster model of chain folding

Hoffman, John D.·1983·Polymer
DOI 10.1016/0032-3861(83)90074-5
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Research works printed but not linked: 43

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  42. If it is assumed that the fraction of gauche states at the various T1 values employed is ‘frozen in’ by sufficiently rapid quenching to a low crystallization temperature, it is possible to predict that the driving force (Δf) at that low temperature will be a function of T1, the larger (Δf) values being associated with the higher T1 values. Then through the relation l∗g≅2σe(Δf) + C2 from nucleation theory, it is readily seen that the smaller initial lamellar thickness l∗g is then associated with the higher T1 value. This is in qualitative accord with the experiments on PE of Cutter et al.19, which involved very rapid quenching to cryogenic temperatures. (It should be noted that Δf ‘with the normal fraction of gauche states is not given by equation (3a) of the text at very low temperatures; see pp. 540–541 of ref. 1.) In the usual ‘slow’ experiment at a normal crystallization temperature, the fraction of gauche states and hence (Δf) would be solely a function of Tx, and no memory effect of T1 would be seen. This is consistent with experiments on PE fractions carried out in Regimes I and II3
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Metadata

Authors
Hoffman, J. D.
Venue
Polymer
Publisher
Elsevier BV
Published
1983-01
Volume
24
Issue
1
Pages
3-26
ISSN
0032-3861 (ISSN-L)
DOI
10.1016/0032-3861(83)90074-5
OpenAlex
W2013531388
Cited by
614
References
0
FWCI
19.10
Type
journal article
Language
en
Open access
closed
Licence
www.elsevier.com/tdm/userlicense/1.0/ (tdm)

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CoChat. (2026). Citation check: Regime III crystallization in melt-crystallized polymers: The variable cluster model of chain folding. https://app.cochat.ai/papers/10.1016/0032-3861(83)90074-5
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Hoffman, J. D. (1983). Regime III crystallization in melt-crystallized polymers: The variable cluster model of chain folding. Polymer. https://doi.org/10.1016/0032-3861(83)90074-5

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