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A novel W-doped Ni-Mg mixed oxide catalyst for CO2 methanation
Open accessAbstract
Novel Ni-W-Mg mixed oxide catalysts (NiWMgOx) were prepared by homogeneous precipitation and attempted for the methanation of CO2. Adding W remarkably promoted the activity with improved stability, anti-CO-poisoning ability and resistance against coke formation compared to the undoped NiMgOx catalyst. The superior reactivity of monodentate formate towards hydrogenation than that of bidentate formate species was identified by DRIFTS analysis and the formation of more active monodentate formate species was indisputably facilitated by W additives, leading to the greatly enhanced catalytic activity. H-2-TPR and CO2-TPD characterization showed that doping W increased the number of stable CO2 adsorption sites and helped in anchoring the Ni sites as a result of strengthened Ni-Mg interaction, both of which were responsible for the enhanced CO2 methanation activity and the improved resistance against sintering. (C) 2016 Elsevier B.V. All rights reserved.
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Recent advances in catalytic hydrogenation of carbon dioxide
Wang, W., Wang, S., Ma, X., & Gong, J. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15008a · Cited by 3,316
Lewis Acido-Basic Interactions between CO 2 and MgO Surface: DFT and DRIFT Approaches
Cornu, D., Guesmi, H., Krafft, J.-M., & Lauron-Pernot, H. (2012) · The Journal of Physical Chemistry C · doi:10.1021/jp211171t · Cited by 203
Cited by
Significant Advances in C1 Catalysis: Highly Efficient Catalysts and Catalytic Reactions
Bao, J., Yang, G., Yoneyama, Y., & Tsubaki, N. (2019) · ACS Catalysis · doi:10.1021/acscatal.8b03924 · Cited by 367
Tuning Zeolite Properties towards CO2 Methanation: An Overview
Bacariza, M. C., Graça, I., Lopes, J. M., & Henriques, C. (2019) · ChemCatChem · doi:10.1002/cctc.201900229 · Cited by 83
Metadata
- Authors
- Yan, Y., Dai, Y., He, H., Yu, Y., & Yang, Y.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2016-11
- Volume
- 196
- Pages
- 108-116
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2374241595
- Cited by
- 216
- References
- 2
- FWCI
- 6.69
- Type
- journal article
- Language
- en
- Open access
- green
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