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Selective reduction of CO2 by conductive MOF nanosheets as an efficient co-catalyst under visible light illumination
Abstract
Abstract Mimicking the natural photosynthesis process, photocatalytic conversion of CO2 has been an ongoing hotspot of scientific research and technology development. A key aspect is the discovery of high potency catalysts for facilitating the multi-electron participated reactions. Herein we successfully demonstrate exfoliated nanosheets from a conductive 2D-MOF Ni3(HITP)2 as an efficient co-catalyst for CO2 reduction in a hybrid photocatalytic system under visible light illumination. By taking advantage of the high conductivity for charge transportation and highly accessible active sites for redox reactions, an excellent selectivity of 97% for deoxygenative CO2 reduction and a high CO yield rate of 3.45 × 104 μmol·g−1 h−1 were achieved with superior stability. This work provides essential insights into future design and development of more effective MOFs-based systems for catalytic CO2 utilization.
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Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013) · Chemical Reviews · doi:10.1021/cr300503r · Cited by 9,590
Recent Advances in Heterogeneous Photocatalytic CO 2 Conversion to Solar Fuels
Li, K., Peng, B., & Peng, T. (2016) · ACS Catalysis · doi:10.1021/acscatal.6b02089 · Cited by 1,355
Cited by
Cocatalysts for Selective Photoreduction of CO2into Solar Fuels
Li, X., Yu, J., Jaroniec, M., & Chen, X. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00400 · Cited by 2,304
Product selectivity of photocatalytic CO2 reduction reactions
Fu, J., Jiang, K., Qiu, X., Yu, J., & Liu, M. (2020) · Materials Today · doi:10.1016/j.mattod.2019.06.009 · Cited by 1,280
Emerging trends in porous materials for CO2capture and conversion
Singh, G., Lee, J., Karakoti, A., Bahadur, R., Yi, J., Zhao, D., AlBahily, K., & Vinu, A. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00075b · Cited by 843
Zhong, W., Sa, R., Li, L., He, Y., Li, L., Bi, J., Zhuang, Z., Yu, Y., & Zou, Z. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b02997 · Cited by 769
Lu, K.-Q., Li, Y.-H., Zhang, F., Qi, M.-Y., Chen, X., Tang, Z.-R., Yamada, Y. M. A., Anpo, M., Conte, M., & Xu, Y.-J. (2020) · Nature Communications · doi:10.1038/s41467-020-18944-1 · Cited by 371
Metadata
- Authors
- Zhu, W., Zhang, C., Li, Q., Xiong, L., Chen, R., Wan, X., Wang, Z., Chen, W., Deng, Z., & Peng, Y.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2018-12
- Volume
- 238
- Pages
- 339-345
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2876685530
- Cited by
- 202
- References
- 2
- FWCI
- 5.32
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhu, W., Zhang, C., Li, Q., Xiong, L., Chen, R., Wan, X., Wang, Z., Chen, W., Deng, Z., & Peng, Y. (2018). Selective reduction of CO2 by conductive MOF nanosheets as an efficient co-catalyst under visible light illumination. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2018.07.024
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