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Electrocatalysis of 5-hydroxymethylfurfural at cobalt based spinel catalysts with filamentous nanoarchitecture in alkaline media
Abstract
Abstract This study reports the activity of cobalt based metal oxide electrode with spinel structure for 5-hydroxymethylfurfural (HMF) oxidation. For that purpose, the Co3O4 and NiCo2O4 electrode with filamentous nanoarchitecture were grown on Ni foam by a hydrothermal method and then characterized by means of SEM, TEM, and XPS analyses. During electrochemical oxidation of HMF, the role of Co3+ in Co3O4 and NiCo2O4 spinel structure was investigated by XANES. The filamentous nanoarchitecture of NiCo2O4 showed 99.6% 5-hydroxymethylfurfural (HMF) conversion efficiency with 90.8% selectivity on 2,5-furandicarboxylic acid (FDCA). The catalyst was successfully recycled up to three times, retaining over 80% of FDCA conversion efficiency. These results demonstrated the potential interest of NiCo2O4 anodic catalyst, prepared via hydrothermal method, for production of high-valued chemical from biomass-derived compounds via electrochemical techniques.
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Opportunities and challenges for a sustainable energy future
Chu, S., & Majumdar, A. (2012) · Nature · doi:10.1038/nature11475 · Cited by 12,550
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
Cited by
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
Yang, Y., & Mu, T. (2021) · Green Chemistry · doi:10.1039/d1gc00914a · Cited by 539
Zhang, N., Zou, Y., Tao, L., Chen, W., Zhou, L., Liu, Z., Zhou, B., Huang, G., Lin, H., & Wang, S. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201908722 · Cited by 523
Lu, Y., Liu, T., Huang, Y.-C., Zhou, L., Li, Y., Chen, W., Yang, L., Zhou, B., Wu, Y., Kong, Z., et al. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c00174 · Cited by 282
Metadata
- Authors
- Kang, M. J., Park, H., Jegal, J., Hwang, S. Y., Kang, Y. S., & Cha, H. G.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2019-03
- Volume
- 242
- Pages
- 85-91
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2895459266
- Cited by
- 228
- References
- 2
- FWCI
- 5.66
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kang, M. J., Park, H., Jegal, J., Hwang, S. Y., Kang, Y. S., & Cha, H. G. (2019). Electrocatalysis of 5-hydroxymethylfurfural at cobalt based spinel catalysts with filamentous nanoarchitecture in alkaline media. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2018.09.087
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