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In situ fabrication of 1D CdS nanorod/2D Ti3C2 MXene nanosheet Schottky heterojunction toward enhanced photocatalytic hydrogen evolution
Abstract
Abstract Benefiting from excellent metallic conductivity, full-spectrum solar energy absorption and rich active sites on the surface, atomically thin two-dimensional transition metal carbide (2D MXene) shows great promise in improving solar-to-hydrogen efficiency and has drawn intense interest in the field of photocatalysis. However, controllable construction of ultrathin 2D MXene-based heterojunction photocatalysts still remains a significant challenge. Herein, one-dimensional (1D) CdS nanorod/2D MXene nanosheet heterojunctions with well-defined nanostructures and strong interfacial coupling are fabricated by in situ assembling solvothermally-generated CdS nanorods on ultrathin Ti3C2 MXene nanosheets. Due to their specific interface characteristics, 1D/2D Schottky heterojunction is capable of providing accelerated charge separation and a lower Schottky barrier for solar-driven hydrogen evolution from water splitting. As expected, the Schottky-based photocatalyst is 7-fold more active in the illuminated hydrogen evolution reaction (HER) than pristine CdS nanorods, implying the synergistic effects between n-type semiconductor CdS and highly conductive 2D Ti3C2 MXene nanosheets.
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Cites
Zhu, X.-D., Xie, Y., & Liu, Y.-T. (2018) · Journal of Materials Chemistry A · doi:10.1039/c8ta08374f · Cited by 208
Cited by
Tang, R., Gong, D., Deng, Y., Xiong, S., Zheng, J., Li, L., Zhou, Z., Su, L., & Zhao, J. (2022) · Journal of Hazardous Materials · doi:10.1016/j.jhazmat.2021.126944 · Cited by 280
Gao, K., Hou, L.-A., An, X., Huang, D., & Yang, Y. (2023) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2022.122150 · Cited by 270
Ti3C2 2D MXene: Recent Progress and Perspectives in Photocatalysis
Tang, R., Xiong, S., Gong, D., Deng, Y., Wang, Y., Su, L., Ding, C., Yang, L., & Liao, C. (2020) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.0c12905 · Cited by 259
Metadata
- Authors
- Xiao, R., Zhao, C., Zou, Z., Chen, Z., Tian, L., Xu, H., Tang, H., Liu, Q., Lin, Z., & Yang, X.
- Venue
- Applied Catalysis B: Environment and Energy
- Publisher
- Elsevier BV
- Published
- 2020-07
- Volume
- 268
- Pages
- 118382
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2985521753
- Cited by
- 621
- References
- 1
- FWCI
- 15.41
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Xiao, R., Zhao, C., Zou, Z., Chen, Z., Tian, L., Xu, H., Tang, H., Liu, Q., Lin, Z., & Yang, X. (2020). In situ fabrication of 1D CdS nanorod/2D Ti3C2 MXene nanosheet Schottky heterojunction toward enhanced photocatalytic hydrogen evolution. Applied Catalysis B: Environment and Energy. https://doi.org/10.1016/j.apcatb.2019.118382
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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