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Promotion of electrocatalytic nitrogen reduction reaction on N-doped porous carbon with secondary heteroatoms
Abstract
Abstract The synergistic effect among dual heteroatoms-doped carbons leads to significantly enhanced electrochemical performance. Herein, with N as the primary dopant, B, F, P, and S as the secondary heteroatoms are introduced into porous carbons respectively to investigate their electrocatalytic nitrogen reduction reaction (NRR) performance. The promoting effect of B, F, P, and S to N-doped carbons for NRR is different from the experimental evolution and analysis. In there, N,B-codoping of porous carbon has the greatest promotional effect in NRR. The electronic structure of these doped carbons determines the electrocatalytic activity. For instance, with the presence of B dopant, the fabricated N-doped materials exhibit a higher content of pyridinic-N. Further systematic and controlled experiments demonstrate that the presence of B element facilitates the formation of B–N bonds, thus boosting NRR activity. From in situ Fourier transform infrared spectroscopic findings, this N,B dual-doped carbons follow the associative mechanism during NRR process.
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Alternative energy technologies
Dresselhaus, M. S., & Thomas, I. L. (2001) · Nature · doi:10.1038/35104599 · Cited by 4,894
Hydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
Cited by
Weng, C., Ren, J., & Yuan, Z. (2020) · ChemSusChem · doi:10.1002/cssc.202000416 · Cited by 342
Self-citationRecent progress in metal–organic frameworks (MOFs) for electrocatalysis
Li, C., Zhang, H., Liu, M., Lang, F.-F., Pang, J., & Bu, X.-H. (2023) · Industrial Chemistry & Materials · doi:10.1039/d2im00063f · Cited by 339
Metadata
- Authors
- Ren, J.-T., Wan, C.-Y., Pei, T.-Y., Lv, X.-W., & Yuan, Z.-Y.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2020-06
- Volume
- 266
- Pages
- 118633
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W2998736407
- Cited by
- 168
- References
- 2
- FWCI
- 5.52
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ren, J.-T., Wan, C.-Y., Pei, T.-Y., Lv, X.-W., & Yuan, Z.-Y. (2020). Promotion of electrocatalytic nitrogen reduction reaction on N-doped porous carbon with secondary heteroatoms. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2020.118633
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