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In situ facile fabrication of Ni(OH)2 nanosheet arrays for electrocatalytic co-production of formate and hydrogen from methanol in alkaline solution
Abstract
Abstract Ni(OH)2 nanosheet arrays are in situ prepared on Ni foam through very straightforward ultrasonication in HCl solution and the following rinsing and drying procedures. Value-added formate and hydrogen could be co-produced by selective oxidation of methanol without carbon dioxide emissions and water reduction over Ni(OH)2 nanosheet arrays bifunctional electrocatalysts. Energy depletion for hydrogen evolution from water could be reduced by integrating with selective methanol oxidation rather than oxygen evolution. The prepared Ni(OH)2 nanosheet arrays exhibits high activity for selective methanol oxidation in alkaline methanol-water solution. It gives a low potential of only 1.36 V (vs. reversible hydrogen electrode) to drive the current density of 100 mA cm−2. The faradaic efficiencies of formate are approximately 100% with the current densities from 10 mA cm−2 to 100 mA cm−2. Moreover, it is easy to separate the anodic and cathodic products without help of any membrane, which greatly simplifies the electrolysis system.
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Opportunities and challenges for a sustainable energy future
Chu, S., & Majumdar, A. (2012) · Nature · doi:10.1038/nature11475 · Cited by 12,550
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
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Recent Advancements in Electrochemical Hydrogen Production via Hybrid Water Splitting
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Toward Electrocatalytic Methanol Oxidation Reaction: Longstanding Debates and Emerging Catalysts
Wang, J., Zhang, B., Guo, W., Wang, L., Chen, J., Pan, H., & Sun, W. (2023) · Advanced Materials · doi:10.1002/adma.202211099 · Cited by 339
Self-citationCuNi Aerogels with Suppressed Water Activation for Efficient Nucleophilic Methanol Electrooxidation
Fang, Q., Ye, S., Zheng, L., Wang, H., Hu, L., Gu, W., Wang, L., Shi, L., & Zhu, C. (2024) · ACS Catalysis · doi:10.1021/acscatal.4c01596 · Cited by 48
Self-citationPdRh bimetallene for energy-saving hydrogen production via methanol electroreforming
Mao, Q., Wang, P., Wang, Z., Xu, Y., Li, X., Wang, L., & Wang, H. (2022) · Applied Materials Today · doi:10.1016/j.apmt.2022.101400 · Cited by 26
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Metadata
- Authors
- Hao, J., Liu, J., Wu, D., Chen, M., Liang, Y., Wang, Q., Wang, L., Fu, X.-Z., & Luo, J.-L.
- Venue
- Applied Catalysis B: Environmental
- Publisher
- Elsevier BV
- Published
- 2021-02
- Volume
- 281
- Pages
- 119510
- ISSN
- 0926-3373 (ISSN-L)
- OpenAlex
- W3082336612
- Cited by
- 270
- References
- 2
- FWCI
- 6.94
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hao, J., Liu, J., Wu, D., Chen, M., Liang, Y., Wang, Q., Wang, L., Fu, X.-Z., & Luo, J.-L. (2021). In situ facile fabrication of Ni(OH)2 nanosheet arrays for electrocatalytic co-production of formate and hydrogen from methanol in alkaline solution. Applied Catalysis B: Environmental. https://doi.org/10.1016/j.apcatb.2020.119510
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