The DOI matches its Crossref record; 46 of the 46 references it cites were found in a registry or an index.
Graphene oxide spontaneous reduction and self-assembly on the zinc metal surface enabling a dendrite-free anode for long-life zinc rechargeable aqueous batteries
Abstract
Abstract Rechargeable aqueous Zn-based batteries are one of the most promising large-scale energy storage devices, benefiting from their eco-friendliness, low cost, high power/energy densities, and safety advantages without using flammable and poisonous organic liquid electrolytes. However, various challenges, such as infinite volume change and growth of dendrites during the electrostripping/electroplating process, lead to low cycling stability (cell shorting) and hinders the application of Zn-based batteries. Herein, a facile and effective approach to reduce graphene oxide (GO) spontaneously by zinc metal is developed and subsequently, the reduced graphene oxide (rGO) is self-assembled to create a layer-by-layer film on the Zn foil surface. This self-assembled, layered rGO on a Zn surface provides a large electroactive area and a soft substrate for Zn electrodeposition, which significantly mitigates Zn dendritic growth by eliminating its driving force. Compared with bare Zn, this composite anode exhibits much lower overpotential (~20 mV at 1 mA cm−2) and excellent long-life cyclability. A full-device with active carbon demonstrates good rate capacity and superior cycling stability. This well-designed anode also provides a useful solution and the possibility of constructing a dendrite-free advanced zinc anode. This is very important to all the zinc-based batteries for grid-scale storage.
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Cited by
Scientific Challenges for the Implementation of Zn-Ion Batteries
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Interfacial Manipulation via In Situ Grown ZnSe Cultivator toward Highly Reversible Zn Metal Anodes
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Metadata
- Authors
- Xia, A., Pu, X., Tao, Y., Liu, H., & Wang, Y.
- Venue
- Applied Surface Science
- Publisher
- Elsevier BV
- Published
- 2019-07
- Volume
- 481
- Pages
- 852-859
- ISSN
- 0169-4332 (ISSN-L)
- OpenAlex
- W2924603060
- Cited by
- 308
- References
- 46
- FWCI
- 13.13
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xia, A., Pu, X., Tao, Y., Liu, H., & Wang, Y. (2019). Graphene oxide spontaneous reduction and self-assembly on the zinc metal surface enabling a dendrite-free anode for long-life zinc rechargeable aqueous batteries. Applied Surface Science. https://doi.org/10.1016/j.apsusc.2019.03.197
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