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Cited by 187Adsorption and biosorption for pollutant removalThermochemical Biomass Conversion ProcessesCoagulation and Flocculation Studies

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Mechanisms and adsorption capacities of hydrogen peroxide modified ball milled biochar for the removal of methylene blue from aqueous solutions

Zhang, Yue, Zheng, Yulin, Yang, Yicheng, Huang, Jinsheng, Zimmerman, Andrew R., Chen, Hao, Hu, Xin, Gao, Bin·2021·Bioresource Technology
DOI 10.1016/j.biortech.2021.125432
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Abstract

In this work, hickory chip biochars developed at distinctive pyrolysis temperatures were ball milled (BMHC) and then post-modified with a 10% hydrogen peroxide (H 2 O 2) solution to obtain a set of novel sorbents (BMHC-H 2 O 2). The specific surface area (SSA) was dramatically increased after ball-milling while the hydroxyl and carboxyl groups on the surface of the biochars were further increased through H 2 O 2 modification. Additionally, thermal stability of the biochar treated with ball-milling was not greatly reduced by H 2 O 2 modification and hydrodynamic radius was decreased. Ball milling enhanced the adsorption efficiency to methylene blue (MB) by the biochar, and this ability was further increased by H 2 O 2 modification, because of the increasing in oxygen-containing functional groups (OCFG) to interact with MB. The rate of MB adsorption to BMHC-H 2 O 2 was faster than that of BMHC, reaching equilibrium after about 6 h. Among adsorbents tested, the 450 °C BMHC-H 2 O 2 had the greatest MB adsorption capacity (310 mg g-1).

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  • Specific surface area of biochar significantly increased after Ball-milling, and hydroxyl and carboxyl groups further increased after H2O2 modification.

    “It was found that the specific surface area (SSA) of biochar significantly increased after Ball-milling, and the hydroxyl groups and carboxyl groups on biochar further increased after the H 2 O2 modification.”

    From Modified biochar: synthesis and mechanism for removal of environmental heavy metals (2022) · cites this paper as Zhang et al. (2021b)

  • BMHCH2O2-450 had the largest sorption capacity for methylene blue (310 mg/g) among tested adsorbents.

    “Among the tested adsorbents, BMHCH 2 O2-450 had the largest sorption capacity for MB (310mg · g -1 )”

    From Modified biochar: synthesis and mechanism for removal of environmental heavy metals (2022) · cites this paper as Zhang et al. (2021b)

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Metadata

Authors
Zhang, Y., Zheng, Y., Yang, Y., Huang, J., Zimmerman, A. R., Chen, H., Hu, X., & Gao, B.
Affiliations
  • University of Florida (US)
  • University of Arkansas at Pine Bluff (US)
  • Nanjing University (CN)
Corresponding author
Gao, Bin
ORCID
Venue
Bioresource Technology
Publisher
Elsevier BV
Published
2021-10
Volume
337
Pages
125432
ISSN
0960-8524 (ISSN-L)
DOI
10.1016/j.biortech.2021.125432
OpenAlex
W3175886863
Cited by
187
References
2
Citations by year
2026: 29 · 2025: 28 · 2024: 43 · 2023: 37 · 2022: 44 · 2021: 5
FWCI
9.61
Type
journal article
Language
en
Open access
closed
Licence
Locations
  • Bioresource Technology (publishedVersion)
  • PubMed (publishedVersion)
Topics
  • Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
  • Physical Sciences › Energy › Fuel Technology › Thermochemical Biomass Conversion Processes
  • Physical Sciences › Environmental Science › Water Science and Technology › Coagulation and Flocculation Studies
Keywords
biochar, ball milling, hydrogen peroxide modification, methylene blue, dye adsorption, pyrolysis temperature, oxygen-containing functional groups, specific surface area, adsorption kinetics, adsorption capacity, wastewater treatment
MeSH terms
Adsorption, Charcoal, Hydrogen Peroxide, Methylene Blue, Water Pollutants, Chemical

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