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One-step synthesis of Co-doped UiO-66 nanoparticle with enhanced removal efficiency of tetracycline: Simultaneous adsorption and photocatalysis
Open accessAbstract
Abstract In this study, a novel recyclable Co-doped UiO-66 nanoparticle was synthesized by a one-step solvothermal method. A high adsorption capacity of 224.1 mg g−1 was obtained by the CoUiO-1 nanoparticle, then the adsorbed tetracycline (TC) molecules could be removed more than 94% of initial concentration under simulative sunlight irradiation. The adsorptive ability and photocatalytic performance of CoUiO-1 nanoparticle were about 7.6 and 6.9 times higher than the pristine UiO-66, respectively. The adsorption capacity of CoUiO-1 nanoparticle was sensitive to adsorbent dosage, coexisting ions, solution pH values and initial TC concentrations. Pseudo-second-order and Freundlich models fitted well with the adsorption process. Thermodynamic study indicated the TC adsorption on CoUiO-1 nanoparticle was a spontaneous and exothermic process. TC photodegradation experiment showed that the Co-doped modification expanded light absorption and facilitated charge separation of UiO-66, which was beneficial to enhance photocatalytic performance. The mechanism of TC photodegradation by Co-doped UiO-66 nanoparticle was investigated. Moreover, a plausible degradation pathway for TC was proposed. The high removal efficiencies of CoUiO-1 nanoparticle were obtained towards real samples including tap water, river water and pharmaceutical wastewater. Therefore, the novel Co-doped MOFs photocatalytic adsorbent showed great potential in wastewater treatment.
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Wu, H. B., Xia, B. Y., Yu, L., Yu, X.-Y., & Lou, X. W. (2015) · Nature Communications · doi:10.1038/ncomms7512 · Cited by 1,434
Cited by
Winarta, J., Shan, B., Mcintyre, S. M., Ye, L., Wang, C., Liu, J., & Mu, B. (2020) · Crystal Growth & Design · doi:10.1021/acs.cgd.9b00955 · Cited by 641
Wang, Y., Rao, L., Wang, P., Shi, Z., & Zhang, L. (2020) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.118308 · Cited by 560
UiO-66 metal–organic frameworks in water treatment: A critical review
Ahmadijokani, F., Molavi, H., Rezakazemi, M., Tajahmadi, S., Bahi, A., Ko, F., Aminabhavi, T. M., Li, J.-R., & Arjmand, M. (2022) · Progress in Materials Science · doi:10.1016/j.pmatsci.2021.100904 · Cited by 559
Du, C., Zhang, Z., Yu, G., Wu, H., Chen, H., Zhou, L., Zhang, Y., Su, Y., Tan, S., Yang, L., et al. (2021) · Chemosphere · doi:10.1016/j.chemosphere.2020.129501 · Cited by 543
Self-citationApplications of water-stable metal-organic frameworks in the removal of water pollutants: A review
Zhang, S., Wang, J., Zhang, Y., Ma, J., Huang, L., Yu, S., Chen, L., Song, G., Qiu, M., & Wang, X. (2021) · Environmental Pollution · doi:10.1016/j.envpol.2021.118076 · Cited by 458
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Metadata
- Authors
- Cao, J., Yang, Z.-H., Xiong, W.-P., Zhou, Y.-Y., Peng, Y.-R., Li, X., Zhou, C.-Y., Xu, R., & Zhang, Y.-R.
- Venue
- Chemical Engineering Journal
- Publisher
- Elsevier BV
- Published
- 2018-12
- Volume
- 353
- Pages
- 126-137
- ISSN
- 1385-8947 (ISSN-L)
- OpenAlex
- W2860293067
- Cited by
- 505
- References
- 1
- FWCI
- 17.60
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Cao, J., Yang, Z.-H., Xiong, W.-P., Zhou, Y.-Y., Peng, Y.-R., Li, X., Zhou, C.-Y., Xu, R., & Zhang, Y.-R. (2018). One-step synthesis of Co-doped UiO-66 nanoparticle with enhanced removal efficiency of tetracycline: Simultaneous adsorption and photocatalysis. Chemical Engineering Journal. https://doi.org/10.1016/j.cej.2018.07.060
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