Accelerated carbonation and structural transformation of blast furnace slag by mechanochemical alkali-activation
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In prior work, mechanochemical processing of industrial waste materials in a CO2-rich atmosphere produced a hydraulic cement paste that incorporated weight percent amounts of CO2 in the form of carbonate minerals.
“In our prior work, we observed that mechano-chemical processing of industrial waste materials in a CO2-rich atmosphere produced a hydraulic cement paste that incorporated weight percent amounts of CO2 in the form of carbonate minerals [17, 18].”
From Mechanochemical formation of highly stable amorphous calcium carbonate in calcium silicates: Potential long-term storage of CO2 in cement (2024) · cites this paper as [17]
ACC as well as network forming and non-bridging carbonate phases were identified in initially prepared material that transformed into crystalline carbonate phases when mixed into a cement paste during hydration reactions.
“Amorphous calcium carbonate (ACC) as well as network forming, and non-bridging carbonate phases were identified in the initially prepared material that transformed into crystalline carbonate phases when mixed into a cement paste during the hydration reactions.”
From Mechanochemical formation of highly stable amorphous calcium carbonate in calcium silicates: Potential long-term storage of CO2 in cement (2024) · cites this paper as [17]
Carbonate minerals can effectively act as hydraulic binder in cement materials formulated with waste materials.
“Previous work has shown that carbonate minerals can effectively act as hydraulic binder in cement materials formulated with waste materials [17, 18, 44-46].”
From Mechanochemical formation of highly stable amorphous calcium carbonate in calcium silicates: Potential long-term storage of CO2 in cement (2024) · cites this paper as [17]
Mechanochemical milling of blast furnace slag in a CO2-rich atmosphere generates metastable carbonate phases with ACC as a major component.
“Mechanochemical milling of blast furnace slag in a CO2 rich atmosphere generates a combination of metastable carbonate phases of which ACC is major component [17].”
From Mechanochemical formation of highly stable amorphous calcium carbonate in calcium silicates: Potential long-term storage of CO2 in cement (2024) · cites this paper as [17]
Cites
Myers, R. J., Bernal, S. A., San Nicolas, R., & Provis, J. L. (2013) · Langmuir · doi:10.1021/la4000473 · Cited by 579 · see citing works
The negative emission potential of alkaline materials
Renforth, P. (2019) · Nature Communications · doi:10.1038/s41467-019-09475-5 · Cited by 403 · see citing works
CO<sub>2</sub> Sequestration Potential of Steel Slags at Ambient Pressure and Temperature
Bonenfant, D., Kharoune, L., Sauve´, S., Hausler, R., Niquette, P., Mimeault, M., & Kharoune, M. (2008) · Industrial & Engineering Chemistry Research · doi:10.1021/ie701721j · Cited by 215 · see citing works
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Vaughn, J. S., Marple, M. A. T., & Mason, H. E. (2024) · Cement and Concrete Research · doi:10.1016/j.cemconres.2023.107413 · Cited by 18 · see citing works
Self-citation
- Authors
- Marple, M. A. T., Koroglu, B., Morrison, K., Crowhurst, J., Balachandra, A., Soroushian, P., & Mason, H. E.
- Affiliations
- Lawrence Livermore National Laboratory (US)
- Metna (United States) (US)
- Corresponding author
- Marple, Maxwell A.T.
- ORCID
- Venue
- Cement and Concrete Research
- Publisher
- Elsevier BV
- Published
- 2022-06
- Volume
- 156
- Pages
- 106760
- ISSN
- 0008-8846 (ISSN-L)
- OpenAlex
- W4220955647
- Cited by
- 57
- References
- 3
- Citations by year
- 2026: 13 · 2025: 12 · 2024: 11 · 2023: 17 · 2022: 4
- FWCI
- 4.82
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Cement and Concrete Research (acceptedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- Funders
- U.S. Department of Energy (DOE-SC0011960, DE-AC52-07NA27344, LLNL-JRNL-811939)
- Topics
- Physical Sciences › Engineering › Civil and Structural Engineering › Concrete and Cement Materials Research
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Physical Sciences › Engineering › Mechanical Engineering › Bauxite Residue and Utilization
- Keywords
- blast furnace slag, alkali activation, mechanochemical milling, CO2 capture, carbonation, low-carbon cement, bicarbonate, calcite, aragonite, gaylussite
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Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
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