Cited by 178Advanced oxidation water treatmentAdvanced Photocatalysis TechniquesWater Treatment and Disinfection

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A critical review on advanced oxidation processes for the removal of trace organic contaminants: A voyage from individual to integrated processes

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Tufail, Arbab, Price, William E., Hai, Faisal I.·2020·Chemosphere

DOI 10.1016/j.chemosphere.2020.127460

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Abstract

Advanced oxidation processes (AOPs), such as photolysis, photocatalysis, ozonation, Fenton process, anodic oxidation, sonolysis, and wet air oxidation, have been investigated extensively for the removal of a wide range of trace organic contaminants (TrOCs). A standalone AOP may not achieve complete removal of a broad group of TrOCs. When combined, AOPs produce more hydroxyl radicals, thus performing better degradation of the TrOCs. A number of studies have reported significant improvement in TrOC degradation efficiency by using a combination of AOPs. This review briefly discusses the individual AOPs and their limitations towards the degradation of TrOCs containing different functional groups. It also classifies integrated AOPs and comprehensively explains their effectiveness for the degradation of a wide range of TrOCs. Integrated AOPs are categorized as UV irradiation based AOPs, ozonation/Fenton process-based AOPs, and electrochemical AOPs. Under appropriate conditions, combined AOPs not only initiate degradation but may also lead to complete mineralization. Various factors can affect the efficiency of integrated processes including water chemistry, the molecular structure of TrCOs, and ions co-occurring in water. For example, the presence of organic ions (e.g., humic acid and fulvic acid) and inorganic ions (e.g., halide, carbonate, and nitrate ions) in water can have a significant impact. In general, these ions either convert to high redox potential radicals upon collision with other reactive species and increase the reaction rates, or may act as radical scavengers and decrease the process efficiency.

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Enhanced Biodegradation of Carbamazepine after UV/H2O2 Advanced Oxidation
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Photocatalytic removal of atrazine using N-doped TiO2 supported on phosphors
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Sonoelectro-Fenton process: A novel hybrid technique for the destruction of organic pollutants in water
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UV Photolysis of Nitrate: Effects of Natural Organic Matter and Dissolved Inorganic Carbon and Implications for UV Water Disinfection
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Reaction kinetics of selected micropollutants in ozonation and advanced oxidation processes
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Phenol degradation using 20, 300 and 520kHz ultrasonic reactors with hydrogen peroxide, ozone and zero valent metals
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Transformation of atrazine, carbamazepine, diclofenac and sulfamethoxazole by low and medium pressure UV and UV/H2O2 treatment
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O3 and O3/H2O2 treatment of sulfonamide and macrolide antibiotics in wastewater
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Photocatalytic degradation of carbamazepine and three derivatives using TiO₂ and ZnO: effect of pH, ionic strength, and natural organic matter.
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Study of the Coalescence of Acoustic Bubbles as a Function of Frequency, Power, and Water-Soluble Additives
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Study of the toxicity of diuron and its metabolites formed in aqueous medium during application of the electrochemical advanced oxidation process “electro-Fenton”
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New treatment of stabilized leachate by ozone/Fenton in the advanced oxidation process
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Ozonation of trimethoprim in aqueous solution: Identification of reaction products and their toxicity
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Biological assessment of bisphenol A degradation in water following direct photolysis and UV advanced oxidation
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Study of the toxicity of sulfamethoxazole and its degradation products in water by a bioluminescence method during application of the electro-Fenton treatment
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Nano-magnetite catalyzed heterogeneous Fenton-like degradation of emerging contaminants carbamazepine and ibuprofen in aqueous suspensions and montmorillonite clay slurries at neutral pH
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Nitrate-induced photodegradation of atenolol in aqueous solution: Kinetics, toxicity and degradation pathways
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Removal of pharmaceuticals using combination of UV/H2O2/O3 advanced oxidation process
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Abatement of the Inhibitory Effect of Chloride Anions on the Photo-Fenton Process
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Investigation of clofibric acid removal by UV/persulfate and UV/chlorine processes: Kinetics and formation of disinfection byproducts during subsequent chlor(am)ination
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Evaluation of a UV-light emitting diodes unit for the removal of micropollutants in water for low energy advanced oxidation processes
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Mechanism considerations for photocatalytic oxidation, ozonation and photocatalytic ozonation of some pharmaceutical compounds in water
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Advanced oxidation of five contaminants in water by UV/TiO2: Reaction kinetics and byproducts identification
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Theory and Fundamentals of Ultrasound
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Mechanism and kinetics of parathion degradation under ultrasonic irradiation
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Combining ozone with UV and H2O2 for the degradation of micropollutants from different origins: lab-scale analysis and optimization
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Authors: Tufail, A., Price, W. E., & Hai, F. I.
Affiliations: University of Wollongong (AU)
Corresponding author: Hai, Faisal I.
ORCID: Tufail, Arbab
Price, William E.
Hai, Faisal I.
Venue: Chemosphere
Publisher: Elsevier BV
Published: 2020-12
Volume: 260
Pages: 127460
ISSN: 0045-6535 (ISSN-L)
DOI: 10.1016/j.chemosphere.2020.127460
OpenAlex: W3038215951
Cited by: 178
References: 233
Citations by year: 2026: 22 · 2025: 41 · 2024: 25 · 2023: 28 · 2022: 29 · 2021: 27 · 2020: 6
FWCI: 1.17
Type: journal article
Language: en
Open access: green
figshare.com
Licence: cc-by
www.elsevier.com/tdm/userlicense/1.0/ (tdm)
www.elsevier.com/legal/tdmrep-license (tdm)
Locations: Chemosphere (publishedVersion)
PubMed (publishedVersion)
Research Online (University of Wollongong) (submittedVersion)
Figshare (submittedVersion, cc-by)
Funders: Higher Education Commission, Pakistan
University of Winchester
Topics: Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
Physical Sciences › Environmental Science › Health, Toxicology and Mutagenesis › Water Treatment and Disinfection
Keywords: advanced oxidation processes, trace organic contaminants, hydroxyl radicals, ozonation, Fenton oxidation, photocatalysis, sonolysis, anodic oxidation, wet oxidation, mineralization, humic acid, fulvic acid, halide ions, carbonate ions, nitrate, radical scavengers, water treatment
MeSH terms: Benzopyrans, Carbonates, Humic Substances, Hydrogen Peroxide, Oxidation-Reduction, Photolysis, Ultraviolet Rays, Water Pollutants, Chemical, Hydroxyl Radical, Water Purification

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A critical review on advanced oxidation processes for the removal of trace organic contaminants: A voyage from individual to integrated processes

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