Cited by 101Adsorption and biosorption for pollutant removalGraphene research and applicationsCoagulation and Flocculation Studies

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Acrylic acid functionalized graphene oxide: High-efficient removal of cationic dyes from wastewater and exploration on adsorption mechanism

Wang, Guanglin, Li, Guangfen, Huan, Yangyang, Hao, Chaoqun, Chen, Wei·2020·Chemosphere

DOI 10.1016/j.chemosphere.2020.127736

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Abstract

A novel p(AA)-g-GO material was prepared by grafting polymerization of acrylic acid (AA) onto graphene oxide (GO) skeleton, presenting efficient removal of dyes from wastewater, because the layer spacing of GO is expanded and successfully introduced numerous polar carboxyl groups. The study revealed a rapid adsorption kinetic process and the adsorption capacity for methylene blue (MB) increases with pH, contact time, initial dye concentration and temperature. The maximum adsorption capacity is about 1448.2 mg/g at 25 °C for MB according to the Langmuir isotherm. More importantly, the adsorbent maintains excellent adsorption capacity after five cycles of adsorption-desorption and has remarkable selective separability for methylene blue/methyl orange mixed solution at pH = 10. Furthermore, the equilibrium adsorption capacities for other cationic dyes as malachite green (MG), basic fuchsin (BF) and rhodamine B (RhB) reached 582.1, 571.7 and 437.1 mg/g, respectively. Additionally, the mechanism analysis indicated that electrostatic interactions, π-π conjugation and hydrogen bonding are the predominant forces for adsorbing cationic dyes. Therefore, p(AA)-g-GO is an outstanding adsorbent and has a potential application prospect in the treatment of dye wastewater.

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Authors: Wang, G., Li, G., Huan, Y., Hao, C., & Chen, W.
Affiliations: Tiangong University (CN)
Corresponding author: Li, Guangfen
ORCID: Wang, Guanglin
Li, Guangfen
Huan, Yangyang
Chen, Wei
Venue: Chemosphere
Publisher: Elsevier BV
Published: 2020-12
Volume: 261
Pages: 127736
ISSN: 0045-6535 (ISSN-L)
DOI: 10.1016/j.chemosphere.2020.127736
OpenAlex: W3043988112
Cited by: 101
References: 44
Citations by year: 2026: 5 · 2025: 11 · 2024: 22 · 2023: 19 · 2022: 19 · 2021: 23 · 2020: 2
FWCI: 4.83
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
www.elsevier.com/legal/tdmrep-license (tdm)
Locations: Chemosphere (publishedVersion)
PubMed (publishedVersion)
Funders: National Natural Science Foundation of China (51378350)
Natural Science Foundation of Tianjin City (17JCTPJC47000)
Topics: Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
Physical Sciences › Materials Science › Materials Chemistry › Graphene research and applications
Physical Sciences › Environmental Science › Water Science and Technology › Coagulation and Flocculation Studies
Keywords: graft copolymerization, cationic dye adsorption, methylene blue, methyl orange, dye wastewater treatment, adsorption mechanism, Langmuir isotherm, adsorbent reusability, electrostatic interactions, π-π conjugation, hydrogen bonding, carboxyl groups
MeSH terms: Acrylates, Adsorption, Cations, Coloring Agents, Graphite, Methylene Blue, Rosaniline Dyes, Water Purification, Wastewater

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Acrylic acid functionalized graphene oxide: High-efficient removal of cationic dyes from wastewater and exploration on adsorption mechanism

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